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We report muon spin relaxation measurements on the superconductor Sr2RuO4 that reveal the spontaneous appearance of an internal magnetic field below the transition temperature: the appearance of such a field indicates that the superconducting state in this material is characterized by the breaking of time-reversal symmetry. These results, combined with other symmetry considerations, suggest that superconductivity in Sr2RuO4 is of p-wave (odd-parity) type, analogous to superfluid 3He.
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By employing a series of experimental techniques, we provide clear evidence that CaPtAs represents a rare example of a noncentrosymmetric superconductor which simultaneously exhibits nodes in the superconducting gap and broken time-reversal symmetry (TRS) in its superconducting state (below $T_c$ $approx$ 1.5 K). Unlike in fully-gapped superconductors, the magnetic penetration depth $lambda(T)$ does not saturate at low temperatures, but instead it shows a $T^2$-dependence, characteristic of gap nodes. Both the superfluid density and the electronic specific heat are best described by a two-gap model comprising of a nodeless gap and a gap with nodes, rather than by single-band models. At the same time, zero-field muon-spin spectra exhibit increased relaxation rates below the onset of superconductivity, implying that TRS is broken in the superconducting state of CaPtAs, hence indicating its unconventional nature. Our observations suggest CaPtAs to be a new remarkable material which links two apparently disparate classes, that of TRS-breaking correlated magnetic superconductors with nodal gaps and the weakly-correlated noncentrosymmetric superconductors with broken TRS, normally exhibiting only a fully-gapped behavior.
Fascinating phenomena have been known to arise from the Dirac theory of relativistic quantum mechanics, which describes high energy particles having linear dispersion relations. Electrons in solids usually have non-relativistic dispersion relations but their quantum excitations can mimic relativistic effects. In topological insulators, electrons have both a linear dispersion relation, the Dirac behavior, on the surface and a non-relativistic energy dispersion in the bulk. Topological phases of matter have attracted much interest, particularly broken-symmetry phases in topological insulator materials. Here, we report by Nb doping that the topological insulator Bi2Se3 can be turned into a bulk type-II superconductor while the Dirac surface dispersion in the normal state is preserved. A macroscopic magnetic ordering appears below the superconducting critical temperature of 3.2 K indicating a spontaneous spin rotation symmetry breaking of the Nb magnetic moments. Even though such a magnetic order may appear at the edge of the superconductor, it is mediated by superconductivity and presents a novel phase of matter which gives rise to a zero-field Hall effect.
The collective mode spectrum of a symmetry-breaking state, such as a superconductor, provides crucial insight into the nature of the order parameter. In this context, we present a microscopic weak-coupling theory for the collective modes of a generic multi-component time-reversal symmetry breaking superconductor, and show that fluctuations in the relative amplitude and phase of the two order parameter components are well-defined underdamped collective modes, even in the presence of nodal quasiparticles. We then demonstrate that these generalized clapping modes can be detected using a number of experimental techniques including ac electronic compressibility measurements, electron energy loss spectroscopy, microwave spectroscopy, and ultrafast THz spectroscopy. Finally, we discuss the implications of our work as a new form of collective mode spectroscopy that drastically expands the number of experimental probes capable of detecting time-reversal symmetry breaking in unconventional superconductors such as Sr$_{text{2}}$RuO$_{text{4}}$, UTe$_{text{2}}$, and moire heterostructures.
Spontaneous time-reversal symmetry (TRS) breaking plays an important role in studying strongly correlated unconventional superconductors. When the superconducting gap functions with different pairing symmetries compete, an Ising ($Z_2$) type symmetry breaking occurs due to the locking of the relative phase $Deltatheta_{12}$ via a second order Josephson coupling. The phase locking can take place even in the normal state in the phase fluctuation regime before the onset of superconductivity. If $Deltatheta_{12}=pmfrac{pi}{2}$, then TRS is broken, otherwise, if $Deltatheta_{12}=0$, or, $pi$, rotational symmetry is broken leading to a nematic state. In both cases, the order parameters possess a 4-fermion structure beyond the scope of mean-field theory. We employ an effective two-component $XY$-model assisted by a renormalization group analysis to address this problem. In addition, a quartetting, or, charge-``4e, superconductivity can also occur above $T_c$. Monte-Carlo simulations are performed and the results are in a good agreement with the renormalization group analysis. Our results provide useful guidance for studying novel symmetry breakings in strongly correlated superconductors.
Superconductivity that spontaneously breaks time-reversal symmetry (TRS) has been found, so far, only in a handful of 3D crystals with bulk inversion symmetry. Here we report an observation of spontaneous TRS breaking in a 2D superconducting system without inversion symmetry: the epitaxial bilayer films of bismuth and nickel. The evidence comes from the onset of the polar Kerr effect at the superconducting transition in the absence of an external magnetic field, detected by the ultrasensitive loop-less fiber-optic Sagnac interferometer. Because of strong spin-orbit interaction and lack of inversion symmetry in a Bi/Ni bilayer, superconducting pairing cannot be classified as singlet or triplet. We propose a theoretical model where magnetic fluctuations in Ni induce superconducting pairing of the dxy = +- idx^2y^2 orbital symmetry between the electrons in Bi. In this model the order parameter spontaneously breaks the TRS and has a non-zero phase winding number around the Fermi surface, thus making it a rare example of a 2D topological superconductor.
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