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Register a new userBose glass and Mott glass of quasiparticles in a doped quantum magnet
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The low-temperature states of bosonic fluids exhibit fundamental quantum effects at the macroscopic scale: the best-known examples are Bose-Einstein condensation (BEC) and superfluidity, which have been tested experimentally in a variety of different systems. When bosons are interacting, disorder can destroy condensation leading to a so-called Bose glass. This phase has been very elusive to experiments due to the absence of any broken symmetry and of a finite energy gap in the spectrum. Here we report the observation of a Bose glass of field-induced magnetic quasiparticles in a doped quantum magnet (Br-doped dichloro-tetrakis-thiourea-Nickel, DTN). The physics of DTN in a magnetic field is equivalent to that of a lattice gas of bosons in the grand-canonical ensemble; Br-doping introduces disorder in the hoppings and interaction strengths, leading to localization of the bosons into a Bose glass down to zero field, where it acquires the nature of an incompressible Mott glass. The transition from the Bose glass (corresponding to a gapless spin liquid) to the BEC (corresponding to a magnetically ordered phase) is marked by a novel, universal exponent governing the scaling on the critical temperature with the applied field, in excellent agreement with theoretical predictions. Our study represents the first, quantitative account of the universal features of disordered bosons in the grand-canonical ensemble.
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We confirm the presence of a mean-field Bose glass in 2D quasicrystalline Bose-Hubbard models. We focus on two models where the aperiodic component is present in different parts of the problem. First, we consider a 2D generalisation of the Aubry-Andre model, where the lattice geometry is that of a square with a quasiperiodic onsite potential. Second, we consider the randomly disordered vertex model, which takes aperiodic tilings with non-crystalline rotational symmetries, and forms lattices from the vertices and lengths of the tiles. For the disordered vertex models, the mean-field Bose glass forms across large ranges of the chemical potential, and we observe no significant differences from the case of a square lattice with uniform random disorder. Small variations in the critical points in the presence of random disorder between quasicrystalline and crystalline lattice geometries can be accounted for by the varying coordination number and the different rotational symmetries present. In the 2D Aubry-Andre model, substantial differences are observed from the usual phase diagrams of crystalline disordered systems. We show that weak modulation lines can be predicted from the underlying potential and may stabilise or suppress the mean-field Bose glass in certain regimes. This results in a lobe-like structure for the mean-field Bose glass in the 2D Aubry-Andre model, which is significantly different from the case of random disorder. Together, the two quasicrystalline models studied in this work show that the mean-field Bose glass phase is present, as expected for 2D quasiperiodic models. However, a quasicrystalline geometry is not sufficient to result in differences from crystalline realisations of the Bose glass, whereas a quasiperiodic form of disorder can result in different physics, as we observe in the 2D Aubry-Andre model.
In this paper we investigate the quantum phase transition from magnetic Bose glass to magnetic Bose-Einstein condensation induced by a magnetic field in NiCl2.4SC(NH2)2 (dichloro-tetrakis-thiourea-Nickel, or DTN), doped with Br (Br-DTN) or site diluted. Quantum Monte Carlo simulations for the quantum phase transition of the model Hamiltonian for Br-DTN, as well as for site-diluted DTN, are consistent with conventional scaling at the quantum critical point and with a critical exponent z verifying the prediction z=d; moreover the correlation length exponent is found to be nu = 0.75(10) and the order parameter exponent to be beta = 0.95(10). We investigate the low-temperature thermodynamics at the quantum critical field of Br-DTN both numerically and experimentally, and extract the power-law behavior of the magnetization and of the specific heat. Our results for the exponents of the power laws, as well as previous results for the scaling of the critical temperature to magnetic ordering with the applied field, are incompatible with the conventional crossover-scaling Ansatz proposed by Fisher et al., [Phys. Rev. B 40, 546 (1989)], but they can all be reconciled within a phenomenological Ansatz in the presence of a dangerously irrelevant operator.
How a Mott insulator develops into a weakly coupled metal upon doping is a central question to understanding various emergent correlated phenomena. To analyze this evolution and its connection to the high-$T_c$ cuprates, we study the single-particle spectrum for the doped Hubbard model using cluster perturbation theory on superclusters. Starting from extremely low doping, we identify a heavily renormalized quasiparticle dispersion that immediately develops across the Fermi level, and a weakening polaronic side band at higher binding energy. The quasiparticle spectral weight roughly grows at twice the rate of doping in the low doping regime, but this rate is halved at optimal doping. In the heavily doped regime, we find both strong electron-hole asymmetry and a persistent presence of Mott spectral features. Finally, we discuss the applicability of the single-band Hubbard model to describe the evolution of nodal spectra measured by angle-resolved photoemission spectroscopy (ARPES) on the single-layer cuprate La$_{2-x}$Sr$_x$CuO$_4$ ($0 le x le 0.15$). This work benchmarks the predictive power of the Hubbard model for electronic properties of high-$T_c$ cuprates.
The competition between spin glass, ferromagnetism and Kondo effect is analysed here in a Kondo lattice model with an inter-site random coupling $J_{ij}$ between the localized magnetic moments given by a generalization of the Mattis model which represents an interpolation between ferromagnetism and a highly disordered spin glass. Functional integral techniques with Grassmann fields have been used to obtain the partition function. The static approximation and the replica symmetric ansatz have also been used. The solution of the problem is presented as a phase diagram giving $T/{J}$ {it versus} $J_K/J$ where $T$ is the temperature, $J_{K}$ and ${J}$ are the strengths of the intrasite Kondo and the intersite random couplings, respectively. If $J_K/{J}$ is small, when temperature is decreased, there is a second order transition from a paramagnetic to a spin glass phase. For lower $T/{J}$, a first order transition appears between the spin glass phase and a region where there are Mattis states which are thermodynamically equivalent to the ferromagnetism. For very low ${T/{J}}$, the Mattis states become stable. On the other hand, it is found as solution a Kondo state for large $J_{K}/{J}$ values. These results can improve the theoretical description of the well known experimental phase diagram of $CeNi_{1-x}Cu_{x}$.
The relaxations of conductivity have been studied in the glassy regime of a strongly disordered two-dimensional electron system in Si after a temporary change of carrier density during the waiting time t_w. Two types of response have been observed: a) monotonic, where relaxations exhibit aging, i.e. dependence on history, determined by t_w and temperature; b) nonmonotonic, where a memory of the sample history is lost. The conditions that separate the two regimes have been also determined.
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