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Register a new userDirectional point-contact Andreev-reflection spectroscopy of Fe-based superconductors: Fermi surface topology, gap symmetry, and electron-boson interaction
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Point-contact Andreev reflection spectroscopy (PCAR) has proven to be one of the most powerful tools in the investigation of superconductors, where it provides information on the order parameter (OP), a fundamental property of the superconducting state. In the past 20 years, successive improvements of the models used to analyze the spectra have continuously extended its capabilities, making it suited to study new superconductors with exotic properties such as anisotropic, nodal and multiple OPs. In Fe-based superconductors, the complex compound- and doping-dependent Fermi surface and the predicted sensitivity of the OP to fine structural details present unprecedent challenges for this technique. Nevertheless, we show here that PCAR measurements in Fe-based superconductors carried out so far have already greatly contributed to our understanding of these materials, despite some apparent inconsistencies that can be overcome if a homogeneous treatment of the data is used. We also demonstrate that, if properly extended theoretical models for Andreev reflection are used, directional PCAR spectroscopy can provide detailed information not only on the amplitude and symmetry of the OPs, but also on the nature of the pairing boson, and even give some hints about the shape of the Fermi surface.
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We report on the results of directional point-contact Andreev-reflection (PCAR) measurements in Ba(Fe_{1-x}Co_x)2As2 single crystals and epitaxial c-axis oriented films with x = 0.08 as well as in Ca(Fe_{1-x}Co_x)2As2 single crystals with x = 0.06. The PCAR spectra are analyzed within the two-band 3D version of the Blonder-Tinkham-Klapwijk model for Andreev reflection we recently developed, and that makes use of an analytical expression for the Fermi surface that mimics the one calculated within the density-functional theory (DFT). The spectra in Ca(Fe_{0.94}Co_{0.06})2As2 unambiguously demonstrate the presence of nodes or zeros in the small gap. In Ba(Fe_{0.92}Co_{0.08})2As2, the ab-plane spectra in single crystals can be fitted by assuming two nodeless gaps, but this model fails to fit the c-axis ones in epitaxial films. All these results are discussed in comparison with recent theoretical predictions about the occurrence of accidental 3D nodes and the presence of hot spots in the gaps of 122 compounds.
We report on a study of the superconducting order parameter in Fe(Te$_{1-x}$Se$_{x}$) thin films (with different Se contents: x=0.3, 0.4, 0.5) by means of point-contact Andreev-reflection spectroscopy (PCARS). The PCARS spectra show reproducible evidence of multiple structures, namely two clear conductance maxima associated to a superconducting gap of amplitude $Delta_E simeq 2.75 k_B T_c$ and additional shoulders at higher energy that, as we show, are the signature of the strong interaction of charge carriers with a bosonic mode whose characteristic energy coincides with the spin-resonance energy. The details of some PCARS spectra at low energy suggest the presence of a smaller and not easily discernible gap of amplitude $Delta_H simeq 1.75 k_B T_c$. The existence of this gap and its amplitude are confirmed by PCARS measurements in Fe(Te$_{1-x}$Se$_{x}$) single crystals. The values of the two gaps $Delta_E$ and $Delta_H$, once plotted as a function of the local critical temperature $T_c^A$, turn out to be in perfect agreement with the results obtained by various experimental techniques reported in literature.
The newly discovered oxypnictide family of superconductors show very high critical temperatures of up to 55K. Whilst there is growing evidence that suggests a nodal order parameter, point contact Andreev reflection spectroscopy can provide crucial information such as the gap value and possibly the number of energy gaps involved. For the oxygen deficient NdFeAsO0.85 with a Tc of 45.5K, we show that there is clearly a gap value at 4.2K that is of the order of 7meV, consistent with previous studies on oxypnictides with lower Tc. Additionally, taking the spectra as a function of gold tip contact pressure reveals important changes in the spectra which may be indicative of more complex physics underlying this structure.
Directional point-contact Andreev-reflection (PCAR) measurements in Ba(Fe1-xCox)2As2 single crystals (Tc=24.5 K) indicate the presence of two superconducting gaps with no line nodes on the Fermi surface. The PCAR spectra also feature additional structures related to the electron-boson interaction, from which the characteristic boson energy Omega_b(T) is obtained, very similar to the spin-resonance energy observed in neutron scattering experiments. Both the gaps and the additional structures can be reproduced within a three-band s+- Eliashberg model by using an electron-boson spectral function peaked at Omega_0 = 12 meV ~ Omega_b(0).
Systematic studies of the NdFeAsOF superconducting energy gap via the point-contact Andreev-reflection (PCAR) spectroscopy are presented. The PCAR conductance spectra show at low temperatures a pair of gap-like peaks at about 4 - 7 mV indicating the superconducting energy gap and in most cases also a pair of humps at around 10 mV. Fits to the s-wave two-gap model of the PCAR conductance allowed to determine two superconducting energy gaps in the system. The energy-gap features however disappear already at T* = 15 to 20 K, much below the particular Tc of the junction under study. At T* a zero-bias conductance (ZBC) peak emerges, which at higher temperatures usually overwhelms the spectrum with intensity significantly higher than the conductance signal at lower temperatures. Possible causes of this unexpected temperature effect are discussed. In some cases the conductance spectra show just a reduced conductance around the zero-bias voltage, the effect persisting well above the bulk transition temperature. This indicates a presence of the pseudogap in the system.
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