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Register a new userFar-from-equilibrium superconductor in fluctuational regime
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Aleksandra Petkovic
Publication date
2011
fields
Physics
and research's language is
English
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We derive Ginzburg-Landau-like action for two-dimensional disordered superconductor under far-from-equilibrium conditions in a fluctuational regime. Then, utilizing it, we calculate fluctuation induced density of states, Maki-Thomson and Aslamazov-Larkin type contributions to the in-plane electrical conductivity. We apply our approach to thin superconducting film sandwiched between a gate and a substrate that have different temperatures and different electrochemical potentials.
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We show that there exist a class of nonequilibrium systems for which a non-equilibrium analog of the Ginzburg-Landau (GL) functional can be constructed and propose the procedure for its derivation. As an example, we consider a small superconductor island of the size less than the coherence length in a stationary nonequlibrium state. We find the GL expansion of the free energy functional of such a system and analyze the dependence of the coefficients of the expansion upon the external drive and the non-equilibrium distribution functions.
Despite extensive work on high-temperature superconductors, the critical behavior of an incipient condensate has so far been studied exclusively under equilibrium conditions. Here, we excite Bi2Sr2CaCu2O8+d with a femtosecond laser pulse and monitor the subsequent nonequilibrium dynamics of the mid-infrared conductivity. Our data allow us to discriminate temperature regimes where superconductivity is either coherent, fluctuating or vanishingly small. Above the transition temperature Tc, we make the striking observation that the relaxation to equilibrium exhibits power-law dynamics and scaling behavior, both for optimally and underdoped superconductors. Our findings can in part be modeled using time-dependent Ginzburg-Landau theory and provide strong indication of universality in systems far from equilibrium.
The quest for new functionalities in quantum materials has recently been extended to non-equilibrium states, which are interesting both because they exhibit new physical phenomena and because of their potential for high-speed device applications. Notable advances have been made in the creation of metastable phases and in Floquet engineering under external periodic driving. In the context of non-equilibrium superconductivity, examples have included the generation of transient superconductivity above the thermodynamic transition temperature, the excitation of coherent Higgs mode oscillations, and the optical control of the interlayer phase in cuprates. Here, we propose theoretically a novel non-equilibrium phenomenon, through which a prompt quench from a metal to a transient superconducting state could induce large oscillations of the order parameter amplitude. We argue that this oscillating mode could act as a source of parametric amplification of the incident radiation. We report experimental results on optically driven K$_3$C$_{60}$ that are consistent with these predictions. The effect is found to disappear when the onset of the excitation becomes slower than the Higgs mode period, consistent with the theory proposed here. These results open new possibilities for the use of collective modes in many-body systems to induce non-linear optical effects.
We perform time resolved photoelectron spectroscopy measurements of optimally doped $tn{Bi}_2tn{Sr}_2tn{CaCu}_2tn{O}_{8+delta}$ (Bi-2212) and $tn{Bi}_2tn{Sr}_{2-x}tn{La}_{x}tn{Cu}tn{O}_{6+delta}$ (Bi-2201). The electrons dynamics show that inelastic scattering by nodal quasiparticles decreases when the temperature is lowered below the critical value of the superconducting phase transition. This drop of electronic dissipation is astonishingly robust and survives to photoexcitation densities much larger than the value sustained by long-range superconductivity. The unconventional behaviour of quasiparticle scattering is ascribed to superconducting correlations extending on a length scale comparable to the inelastic path. Our measurements indicate that strongly driven superconductors enter in a regime without phase coherence but finite pairing amplitude. The latter vanishes near to the critical temperature and has no evident link with the pseudogap observed by Angle Resolved Photoelectron Spectroscopy (ARPES).
The control of non-equilibrium phenomena in complex solids is an important research frontier, encompassing new effects like light induced superconductivity. Here, we show that coherent optical excitation of molecular vibrations in the organic conductor K3C60 can induce a non-equilibrium state with the optical properties of a superconductor. A transient gap in the real part of the optical conductivity and a low-frequency divergence of the imaginary part are measured for base temperatures far above equilibrium Tc=20 K. These findings underscore the role of coherent light fields in inducing emergent order.
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