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Register a new userQuasiparticles dynamics in high-temperature superconductors far from equilibrium: an indication of pairing amplitude without phase coherence
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We perform time resolved photoelectron spectroscopy measurements of optimally doped $tn{Bi}_2tn{Sr}_2tn{CaCu}_2tn{O}_{8+delta}$ (Bi-2212) and $tn{Bi}_2tn{Sr}_{2-x}tn{La}_{x}tn{Cu}tn{O}_{6+delta}$ (Bi-2201). The electrons dynamics show that inelastic scattering by nodal quasiparticles decreases when the temperature is lowered below the critical value of the superconducting phase transition. This drop of electronic dissipation is astonishingly robust and survives to photoexcitation densities much larger than the value sustained by long-range superconductivity. The unconventional behaviour of quasiparticle scattering is ascribed to superconducting correlations extending on a length scale comparable to the inelastic path. Our measurements indicate that strongly driven superconductors enter in a regime without phase coherence but finite pairing amplitude. The latter vanishes near to the critical temperature and has no evident link with the pseudogap observed by Angle Resolved Photoelectron Spectroscopy (ARPES).
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Despite extensive work on high-temperature superconductors, the critical behavior of an incipient condensate has so far been studied exclusively under equilibrium conditions. Here, we excite Bi2Sr2CaCu2O8+d with a femtosecond laser pulse and monitor the subsequent nonequilibrium dynamics of the mid-infrared conductivity. Our data allow us to discriminate temperature regimes where superconductivity is either coherent, fluctuating or vanishingly small. Above the transition temperature Tc, we make the striking observation that the relaxation to equilibrium exhibits power-law dynamics and scaling behavior, both for optimally and underdoped superconductors. Our findings can in part be modeled using time-dependent Ginzburg-Landau theory and provide strong indication of universality in systems far from equilibrium.
Although initially quite controversial, it has been widely accepted that the Cooper pairs in optimally doped cuprate superconductors have predominantly dx2-y2 wavefunction symmetry. The controversy has now shifted to whether the high-Tc pairing symmetry changes away from optimal doping. Here we present phase-sensitive tricrystal experiments on three cuprate systems: Y0.7Ca0.3Ba2Cu3O7-x (Ca-doped Y-123), La2-xSrxCuO4 (La-214) and Bi2Sr2CaCu2O8+x (Bi-2212),with doping levels covering the underdoped, optimal and overdoped regions. Our work implies that time-reversal invariant, predominantly dx2-y2 pairing symmetry is robust over a large variation in doping, and underscores the important role of on-site Coulomb repulsion in the making of high-temperature superconductivity.
Within the phase fluctuation picture for the pseudogap state of a high-$T_{c}$ superconductor, we incorporate the phase fluctuations generated by the classical XY model with the Bogoliubov-de Gennes formalism utilizing a field-theoretical method. This picture delineates the inhomogeneous characteristics of local order parameters observed in high-$T_{c}$ superconductors above $T_{c}$. We also compute the local density of states near a non-magnetic impurity with a strong scattering potential. The resonance peak smoothly evolves as temperature increases through $T_{c}$ without showing any sudden broadening, which is consistent with recent experimental findings.
Along with some other researches we have realised that the true origin of high-temperature superconductivity should be found in the strong Coulomb repulsion combined with a significant electronphonon interaction. Both interactions are strong (on the order of 1 eV) compared with the low Fermi energy of doped carries which makes the conventional BCS-Eliashberg theory inapplicable in cuprates and related doped insulators. Based on our recent analytical and numerical results I argue that high-temperature superconductivity from repulsion is impossible for any strength of the Coulomb interaction. Major steps of our alternative polaronic theory are outlined starting from the generic Hamiltonian with the unscreened (bare) Coulomb and electron-phonon interactions accounting for critical temperatures of high-temperature superconductors without any adjustable parameters.
The pairing symmetry of the newly proposed cobalt high temperature (high-$T_c$) superconductors formed by vertex shared cation-anion tetrahedral complexes is studied by the methods of mean field, random phase approximation (RPA) and functional renormalization group (FRG) analysis. The results of all these methods show that the $d_{x^2-y^2}$ pairing symmetry is robustly favored near half filling. The RPA and FRG methods, which are valid in weak interaction regions, predict that the superconducting state is also strongly orbital selective, namely the $d_{x^2-y^2}$ orbital that has the largest density near half filling among the three $t_{2g}$ orbitals dominates superconducting pairing. These results suggest that the new materials, if synthesized, can provide indisputable test to high-$T_c$ pairing mechanism and the validity of different theoretical methods.
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