No Arabic abstract
We theoretically investigate signatures of stimulated emission at the single photon level for a two-level atom interacting with a one-dimensional light field. We consider the transient regime where the atom is initially excited, and the steady state regime where the atom is continuously driven with an external pump. The influence of pure dephasing is studied, clearly showing that these effects can be evidenced with state of the art solid state devices. We finally propose a scheme to demonstrate the stimulation of one optical transition by monitoring another one, in three-level one-dimensional atoms.
Solid state quantum emitters have shown strong potential for applications in quantum information, but spectral inhomogeneity of these emitters poses a significant challenge. We address this issue in a cavity-quantum dot system by demonstrating cavity-stimulated Raman spin flip emission. This process avoids populating the excited state of the emitter and generates a photon that is Raman shifted from the laser and enhanced by the cavity. The emission is spectrally narrow and tunable over a range of at least 125 GHz, which is two orders of magnitude greater than the natural linewidth. We obtain the regime in which the Raman emission is spin-dependent, which couples the photon to a long-lived electron spin qubit. This process can enable an efficient, tunable source of indistinguishable photons and deterministic entanglement of distant spin qubits in a photonic crystal quantum network.
Stimulated emission is the process fundamental to laser operation, thereby producing coherent photon output. Despite negatively-charged nitrogen-vacancy (NV$^-$) centres being discussed as a potential laser medium since the 1980s, there have been no definitive observations of stimulated emission from ensembles of NV$^-$ to date. Reasons for this lack of demonstration include the short excited state lifetime and the occurrence of photo-ionisation to the neutral charge state by light around the zero-phonon line. Here we show both theoretical and experimental evidence for stimulated emission from NV$^-$ states using light in the phonon-sidebands. Our system uses a continuous wave pump laser at 532 nm and a pulsed stimulating laser that is swept across the phononic sidebands of the NV$^-$. Optimal stimulated emission is demonstrated in the vicinity of the three-phonon line at 700 nm. Furthermore, we show the transition from stimulated emission to photoionisation as the stimulating laser wavelength is reduced from 700nm to 620 nm. While lasing at the zero-phonon line is suppressed by ionisation, our results open the possibility of diamond lasers based on NV centres, tuneable over the phonon-sideband. This broadens the applications of NV magnetometers from single centre nanoscale sensors to a new generation of ultra-precise ensemble laser sensors, which exploit the contrast and signal amplification of a lasing system.
Single-photon stimulated four wave mixing (StFWM) processes have great potential for photonic quantum information processing, compatible with optical communication technologies and integrated optoelectronics. In this paper, we demonstrate single-photon StFWM process in a piece of optical fiber, with seeded photons generated by spontaneous four wave mixing process (SpFWM). The effect of the single-photon StFWM is confirmed by time-resolved four-photon coincidence measurement and variation of four-photon coincidence counts under different seed-pump delays. According to the experiment results, the potential performance of quantum cloning machine based on the process is analyzed.
The photon statistics of CdSe/CdS dot-in-rods nanocrystals is studied with a method involving post-selection of the photon detection events based on the photoluminescence count rate. We show that flickering between two states needs to be taken into account to interpret the single-photon emission properties. With post-selection we are able to identify two emitting states: the exciton and the charged exciton (trion), characterized by different lifetimes and different second order correlation functions. Measurements of the second order autocorrelation function at zero delay with post- selection shows a degradation of the single photon emission for CdSe/CdS dot-in-rods in a charged state that we explain by deriving the neutral and charged biexciton quantum yields.
Single photon detection is a requisite technique in quantum-optics experiments in both the optical and the microwave domains. However, the energy of microwave quanta are four to five orders of magnitude less than their optical counterpart, making the efficient detection of single microwave photons extremely challenging. Here, we demonstrate the detection of a single microwave photon propagating through a waveguide. The detector is implemented with an impedance-matched artificial $Lambda$ system comprising the dressed states of a driven superconducting qubit coupled to a microwave resonator. We attain a single-photon detection efficiency of $0.66 pm 0.06$ with a reset time of $sim 400$~ns. This detector can be exploited for various applications in quantum sensing, quantum communication and quantum information processing.