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Terahertz (THz) waves have been significantly developed in the last fifteen years because of their great potential for applications in industrial and scientific communities1,2. The unique properties of THz waves as transparency for numerous materials and strong absorption for water-based materials are expected to broadly impact biosensing3 such as medical imaging4, chemical identifications5, and DNA recognition6. In particular, for accessing information within a scale comparable to the cell size where interactions between cell membrane and other organelle structures occur, micron size spatial resolution is required. Due to the large wavelength, however, the joint capability of THz near-field imaging with real-time acquisition, which is a highly desirable ability for observing real-time changes of in vivo sample, remains undone. Here, we report a real-time THz near-field microscope with a high dynamic range that can capture images of a 370 x 740 {mu}m2 area at 35 frames per second. We achieve high spatial resolution on a large area by combining two novel techniques: THz pulse generation by tilted-pulse-front excitation7 and electro-optic (EO) balanced imaging detection using a thin crystal. To demonstrate the microscope capability, we reveal the field enhancement at the gap position of a dipole antenna after the irradiation of a THz pulse. Our results are the first demonstration of a direct quantification of a 2-dimensional subwavelength THz electric field taken in real-time.
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Imaging applications in the terahertz (THz) frequency range are severely restricted by diffraction. Near-field scanning probe microscopy is commonly employed to enable mapping of the THz electromagnetic fields with sub-wavelength spatial resolution, allowing intriguing scientific phenomena to be explored such as charge carrier dynamics in nanostructures and THz plasmon-polaritons in novel 2D materials and devices. High-resolution THz imaging, so far, has been relying predominantly on THz detection techniques that require either an ultrafast laser or a cryogenically-cooled THz detector. Here, we demonstrate coherent near-field imaging in the THz frequency range using a room-temperature nanodetector embedded in the aperture of a near-field probe, and an interferometric optical setup driven by a THz quantum cascade laser (QCL). By performing phase-sensitive imaging of strongly confined THz fields created by plasmonic focusing we demonstrate the potential of our novel architecture for high-sensitivity coherent THz imaging with sub-wavelength spatial resolution.
A proof of concept for high speed near-field imaging with sub-wavelength resolution using SLM is presented. An 8 channel THz detector array antenna with an electrode gap of 100 um and length of 5 mm is fabricated using the commercially available GaAs semiconductor substrate. Each array antenna can be excited simultaneously by spatially reconfiguring the optical probe beam and the THz electric field can be recorded using 8 channel lock-in amplifiers. By scanning the probe beam along the length of the array antenna, a 2D image can be obtained with amplitude, phase and frequency information.
Due to its fast and high resolution characteristics, dual-comb spectroscopy has attracted an increasing amount of interest since its first demonstration. In the terahertz frequency range where abundant absorption lines (finger prints) of molecules are located, multiheterodyne spectroscopy that employs the dual-comb technique shows an advantage in real-time spectral detection over the traditional Fourier transform infrared or time domain spectroscopies. Here, we demonstrate compact terahertz dual-comb spectroscopy based on quantum cascade lasers (QCLs). In our experiment, two free-running QCLs generate approximately 120 GHz wide combs centered at 4.2 THz, with slightly different repetition frequencies. We observe that $sim$490 nW terahertz power coupling of one laser into the other suffices for laser-self-detecting the dual-comb spectrum that is registered by a microwave spectrum analyzer. Furthermore, we demonstrate practical terahertz transmission dual-comb spectroscopy with our device, by implementing a short air path at room temperature. Spectra are shown of semiconductor samples and of moist air, the latter allowing rapid monitoring of the relative humidity. Our devices should be readily extendable to perform imaging, microscopy and near-field microscopy in the terahertz regime.
We present theoretical formulation and experimental demonstration of a novel technique for the fast compression-less terahertz imaging based on the broadband Fourier optics. The technique exploits k-vector/frequency duality in Fourier optics which allows using a single-pixel detector to perform angular scan along a circular path, while the broadband spectrum is used to scan along the radial dimension in Fourier domain. The proposed compression-less image reconstruction technique (hybrid inverse transform) requires only a small number of measurements that scales linearly with the image linear size, thus promising real-time acquisition of high-resolution THz images. Additionally, our imaging technique handles equally well and on the equal theoretical footing the amplitude contrast and the phase contrast images, which makes this technique useful for many practical applications. A detailed analysis of the novel technique advantages and limitations is presented, as well as its place among other existing THz imaging techniques is clearly identified
Excitation of antiferromagnetic spin waves in HoFeO$_{3}$ crystal combined with a split ring resonator (SRR) is studied using terahertz (THz) electromagnetic pulses. The magnetic field in the vicinity of the SRR induced by the incident THz electric field component excites and the Faraday rotation of the polarization of a near-infrared probe pulse directly measures oscillations that correspond to the antiferromagnetic spin resonance mode. The good agreement of the temperature-dependent magnetization dynamics with the calculation using the two-lattice Landau-Lifshitz-Gilbert equation confirms that the spin wave is resonantly excited by the THz magnetic near-field enhanced at the LC resonance frequency of the SRR, which is 20 times stronger than the incident magnetic field.
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