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Register a new userSupersolid Polar Molecules beyond Pairwise Interactions
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We explore the phase diagram of ultracold bosonic polar molecules confined to a planar optical lattice of triangular geometry. External static electric and microwave fields can be employed to tune the effective interactions between the polar molecules into a regime of extended two- and three-body repulsions of comparable strength, leading to a rich quantum phase diagram. In addition to various solid phases, an extended supersolid phase is found to persist deep into the three-body dominated regime. While three-body interactions break particle-hole symmetry explicitly, a characteristic supersolid-supersolid quantum phase transition is observed, which indicates the restoration of particle-hole symmetry at half-filling. We revisit the spatial structure of the supersolid at this filling, regarding the existence of a further supersolid phase with three inequivalent sublattices, and provide evidence that this state is excluded also at finite temperatures.
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We show that s-wave scattering resonances induced by dipolar interactions in a polar molecular gas have a universal large and positive effective range, which is very different from Feshbach resonances realized in cold atoms before, where the effective range is either negligible or negative. Such a difference has important consequence in many-body physics. At high temperature regime, a positive effective range gives rise to stronger repulsive interaction energy for positive scattering length, and weaker attractive interaction energy for negative scattering length. While at low-temperatures, we study polaron problem formed by single impurity molecule, and we find that the polaron binding energy increases at the BEC side and decreases at the BCS side. All these effects are in opposite to narrow Feshbach resonances where the effective range is negative.
We design dipolar quantum many-body Hamiltonians that will facilitate the realization of exotic quantum phases under current experimental conditions achieved for polar molecules. The main idea is to modulate both single-body potential barriers and two-body dipolar interactions on a spatial scale of tens of nanometers to strongly enhance energy scales and, therefore, relax temperature requirements for observing new quantum phases of engineered many-body systems. We consider and compare two approaches. In the first, nanoscale barriers are generated with standing wave optical light fields exploiting optical nonlinearities. In the second, static electric field gradients in combination with microwave dressing are used to write nanostructured spatial patterns on the induced electric dipole moments, and thus dipolar interactions. We study the formation of inter-layer and interface bound states of molecules in these configurations, and provide detailed estimates for binding energies and expected losses for present experimental setups.
This paper reviews recent advances in the study of strongly interacting systems of dipolar molecules. Heteronuclear molecules feature large and tunable electric dipole moments, which give rise to long-range and anisotropic dipole-dipole interactions. Ultracold samples of dipolar molecules with long-range interactions offer a unique platform for quantum simulations and the study of correlated many-body physics. We provide an introduction to the physics of dipolar quantum gases, both electric and magnetic, and summarize the multipronged efforts to bring dipolar molecules into the quantum regime. We discuss in detail the recent experimental progress in realizing and studying strongly interacting systems of polar molecules trapped in optical lattices, with particular emphasis on the study of interacting spin systems and non-equilibrium quantum magnetism. Finally, we conclude with a brief discussion of the future prospects for studies of strongly interacting dipolar molecules.
We demonstrate a scheme for direct absorption imaging of an ultracold ground-state polar molecular gas near quantum degeneracy. A challenge in imaging molecules is the lack of closed optical cycling transitions. Our technique relies on photon shot-noise limited absorption imaging on a strong bound-bound molecular transition. We present a systematic characterization of this imaging technique. Using this technique combined with time-of-flight (TOF) expansion, we demonstrate the capability to determine momentum and spatial distributions for the molecular gas. We anticipate that this imaging technique will be a powerful tool for studying molecular quantum gases.
Quantum states with long-lived coherence are essential for quantum computation, simulation and metrology. The nuclear spin states of ultracold molecules prepared in the singlet rovibrational ground state are an excellent candidate for encoding and storing quantum information. However, it is important to understand all sources of decoherence for these qubits, and then eliminate them, in order to reach the longest possible coherence times. Here, we fully characterise the dominant mechanisms for decoherence of a storage qubit in an optically trapped ultracold gas of RbCs molecules using high-resolution Ramsey spectroscopy. Guided by a detailed understanding of the hyperfine structure of the molecule, we tune the magnetic field to where a pair of hyperfine states have the same magnetic moment. These states form a qubit, which is insensitive to variations in magnetic field. Our experiments reveal an unexpected differential tensor light shift between the states, caused by weak mixing of rotational states. We demonstrate how this light shift can be eliminated by setting the angle between the linearly polarised trap light and the applied magnetic field to a magic angle of $arccos{(1/sqrt{3})}approx55^{circ}$. This leads to a coherence time exceeding 6.9 s (90% confidence level). Our results unlock the potential of ultracold molecules as a platform for quantum computation.
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