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Register a new userChemistry in Disks. III. -- Photochemistry and X-ray driven chemistry probed by the ethynyl radical (CCH) in DM Tau, LkCa 15, and MWC 480
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Authors
Th. Henning
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We studied several representative circumstellar disks surrounding the Herbig Ae star MWC 480 and the T Tauri stars LkCa 15 and DM Tau at (sub-)millimeter wavelengths in lines of CCH. Our aim is to characterize photochemistry in the heavily UV-irradiated MWC 480 disk and compare the results to the disks around cooler T Tauri stars. We detected and mapped CCH in these disks with the IRAM Plateau de Bure Interferome- ter in the C- and D-configurations in the (1-0) and (2-1) transitions. Using an iterative minimization technique, the CCH column densities and excitation conditions are con- strained. Very low excitation temperatures are derived for the T Tauri stars. These values are compared with the results of advanced chemical modeling, which is based on a steady-state flared disk structure with a vertical temperature gradient, and a gas- grain chemical network with surface reactions. Both model and observations suggest that CCH is a sensitive tracer of the X-ray and UV irradiation. The predicted radial dependency and source to source variations of CCH column densities qualitatively agree with the observed values, but the predicted column densities are too low by a factor of several. The chemical model fails to reproduce high concentrations of CCH in very cold disk midplane as derived from the observed low excitation condition for both the (1-0) and (2-1) transitions.
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Aims: To constrain the ionization fraction in protoplanetary disks, we present new high-sensitivity interferometric observations of N$_2$H$^+$ in three disks surrounding DM Tau, LkCa 15, and MWC 480. Methods: We used the IRAM PdBI array to observe the N$_2$H$^+$ J=1-0 line and applied a $chi^2$-minimization technique to estimate corresponding column densities. These values are compared, together with HCO$^+$ column densities, to results of a steady-state disk model with a vertical temperature gradient coupled to gas-grain chemistry. Results: We report two dhp detections for LkCa 15 and DM Tau at the $5 sigma$ level and an upper limit for MWC 480. The column density derived from the data for LkCa 15 is much lower than previously reported. The [N$_2$H$^+$/HCO$^+$] ratio is on the order of 0.02--0.03. So far, HCO$^+$ remains the most abundant observed molecular ion in disks. Conclusions: All the observed values generally agree with the modelled column densities of disks at an evolutionary stage of a few million years (within the uncertainty limits), but the radial distribution of the molecules is not reproduced well. The low inferred concentration of N$_2$H$^+$ in three disks around low-mass and intermediate-mass young stars implies that this ion is not a sensitive tracer of the overall disk ionization fraction.
Context. Several sulfur-bearing molecules are observed in the interstellar medium and in comets, in strong contrast to protoplanetary disks where only CS, H$_2$CS and SO have been detected so far. Aims. We combine observations and chemical models to constrain the sulfur abundances and their sensitivity to physical and chemical conditions in the DM Tau protoplanetary disk. Methods. We obtained $0.5^{}$ ALMA observations of DM Tau in Bands 4 and 6 in lines of CS, SO, SO$_2$, OCS, CCS, H$_2$CS and H$_2$S, achieving a $sim 5$ mJy sensitivity. Using the non-LTE radiative transfer code RADEX and the forward-modeling tool DiskFit, disk-averaged CS column densities and upper limits for the other species were derived. Results. Only CS was detected with a derived column density of $sim 2-6 times 10^{12}$ cm$^{-2}$. We report a first tentative detection of SO$_2$ in DM Tau. The upper limits range between $sim 10^{11}$ and $10^{14}$ cm$^{-2}$ for the other S-bearing species. The best-fit chemical model matching these values requires a gas-phase C/O ratio of > 1 at $r sim 50-100$ au. With chemical modeling we demonstrate that sulfur-bearing species could be robust tracers of the gas-phase C/O ratio, surface reaction rates, grain size and UV intensities. Conclusions. The lack of detections of a variety of sulfur-bearing molecules in DM Tau other than CS implies a dearth of reactive sulfur in the gas phase, either through efficient freeze-out or because most of the elemental sulfur is in other large species, as found in comets. The inferred high CS/SO and CS/SO$_2$ ratios require a non-solar C/O gas-phase ratio of > 1, consistent with the recent observations of hydrocarbon rings in DM Tau. The stronger depletion of oxygen-bearing S-species compared to CS is likely linked to the low observed abundances of gaseous water in DM Tau and points to a removal mechanism of oxygen from the gas.
We study the content in S-bearing molecules of protoplanetary disks around low-mass stars. We used the new IRAM 30-m receiver EMIR to perform simultaneous observations of the $1_{10}-1_{01}$ line of H$_2$S at 168.8 GHz and $2_{23}-1_{12}$ line of SO at 99.3 GHz. We compared the observational results with predictions coming from the astrochemical code NAUTILUS, which has been adapted to protoplanetary disks. The data were analyzed together with existing CS J=3-2 observations. We fail to detect the SO and H$_2$S lines, although CS is detected in LkCa15, DM,Tau, and GO,Tau but not in MWC,480. However, our new upper limits are significantly better than previous ones and allow us to put some interesting constraints on the sulfur chemistry. Our best modeling of disks is obtained for a C/O ratio of 1.2, starting from initial cloud conditions of H density of $2times 10^5$ cm$^{-3}$ and age of $10^6$ yr. The results agree with the CS data and are compatible with the SO upper limits, but fail to reproduce the H$_2$S upper limits. The predicted H$_2$S column densities are too high by at least one order of magnitude. H$_2$S may remain locked onto grain surfaces and react with other species, thereby preventing the desorption of H$_2$S.
We present resolved Plateau de Bure Array observations of DM Tau in lines of HCO+ (3-2), (1-0) and DCO+ (3-2). A power-law fitting approach allowed a derivation of column densities of these two molecules. A chemical inner hole of ~50 AU was found in both HCO+ and DCO+ with DCO+ emission extending to only 450 AU. An isotopic ratio of R_D = N(DCO+) / N(HCO+) was found to range from 0.1 at 50 AU and 0.2 at 450 AU. Chemical modeling allowed an exploration of the sensitivity of these molecular abundances to physical parameters out with temperature, finding that X-rays were the domination ionization source in the HCO+ molecular region and that R_D also is sensitive to the CO depletion. The ionization fraction, assuming a steady state system, was found to be x(e-) ~ 10$^{-7}$. Modeling suggests that HCO+ is the dominant charged molecule in the disk but its contribution to ionization fraction is dwarfed by atmoic ions such as C+, S+ and H+.
H$_2$CO ice on dust grains is an important precursor of complex organic molecules (COMs). H$_2$CO gas can be readily observed in protoplanetary disks and may be used to trace COM chemistry. However, its utility as a COM probe is currently limited by a lack of constraints on the relative contributions of two different formation pathways: on icy grain-surfaces and in the gas-phase. We use archival ALMA observations of the resolved distribution of H$_2$CO emission in the disk around the young low-mass star DM Tau to assess the relative importance of these formation routes. The observed H$_2$CO emission has a centrally peaked and radially broad brightness profile (extending out to 500 AU). We compare these observations with disk chemistry models with and without grain-surface formation reactions, and find that both gas and grain-surface chemistry are necessary to explain the spatial distribution of the emission. Gas-phase H$_2$CO production is responsible for the observed central peak, while grain-surface chemistry is required to reproduce the emission exterior to the CO snowline (where H$_2$CO mainly forms through the hydrogenation of CO ice before being non-thermally desorbed). These observations demonstrate that both gas and grain-surface pathways contribute to the observed H$_2$CO in disks, and that their relative contributions depend strongly on distance from the host star.
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