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On-line Excited-State Laser Spectroscopy of Trapped Short-Lived Ra$^+$ Ions

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 Added by Oscar Versolato
 Publication date 2010
  fields Physics
and research's language is English




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As an important step towards an atomic parity violation experiment in one single trapped Ra$^+$ ion, laser spectroscopy experiments were performed with on-line produced short-lived $^{212,213,214}$Ra$^+$ ions. The isotope shift of the $6,^2$D$_{3/2}$,-,$7,^2$P$_{1/2}$ and $6,^2$D$_{3/2}$,-,$7,^2$P$_{3/2}$ transitions and the hyperfine structure constant of the $7,^2$S$_{1/2}$ and $6,^2$D$_{3/2}$ states in $^{213}$Ra$^+$ were measured. These values provide a benchmark for the required atomic theory. A lower limit of $232(4)$ ms for the lifetime of the metastable $6,^2$D$_{5/2}$ state was measured by optical shelving.



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Laser spectroscopy of short-lived radium isotopes in a linear Paul trap has been performed. The isotope shifts of the $6d,^2$D$_{3/2},$ - $7p,^2$P$_{1/2},$ transition in $^{209-214}$Ra$^+$ were measured, which are sensitive to the short range part of the atomic wavefunctions. The results are essential experimental input for improving the precision of atomic structure calculation. This is indispensable for parity violation in Ra$^+$ aiming at the determination of the weak mixing angle.
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Laser spectroscopic studies on minute samples of exotic radioactive nuclei require very efficient experimental techniques. In addition, high resolving powers are required to allow extraction of nu- clear structure information. Here we demonstrate that by using weak atomic transitions, resonance laser ionization spectroscopy is achieved with the required high efficiency (1-10%) and precision (linewidths of tens of MHz). We illustrate experimentally and through the use of simulations how the narrow experimental linewidths are achieved and how distorted resonance ionization spec- troscopy lineshapes can be avoided. The role of the delay of the ionization laser pulse with respect to the excitation laser pulse is crucial: the use of a delayed ionization step permits the best resolving powers and lineshapes. A high efficiency is maintained if the intermediate level has a lifetime that is at least of the order of the excitation laser pulse width. A model that describes this process re- produces well the observed features and will help to optimize the conditions for future experiments.
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