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Momentum-Resolved Landau-Level Spectroscopy of Dirac Surface State in Bi2Se3

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 Added by Tetsuo Hanaguri
 Publication date 2010
  fields Physics
and research's language is English




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We investigate Dirac fermions on the surface of the topological insulator Bi2Se3 using scanning tunneling spectroscopy. Landau levels (LLs) are observed in the tunneling spectra in a magnetic field. In contrast to LLs of conventional electrons, a field independent LL appears at the Dirac point, which is a hallmark of Dirac fermions. A scaling analysis of LLs based on the Bohr-Sommerfeld quantization condition allowed us to determine the dispersion of the surface band. Near the Fermi energy, fine peaks mixed with LLs appear in the spectra, which may be responsible for the anomalous magneto-fingerprint effect [J. G. Checkelsky et al., Phys. Rev. Lett. 103, 246601 (2009)].



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Massless Dirac electrons in condensed matter have attracted considerable attention. Unlike conventional electrons, Dirac electrons are described in the form of two-component wave functions. In the surface state of topological insulators, these two components are associated with the spin degrees of freedom, hence governing the magnetic properties. Therefore, the observation of the two-component wave function provides a useful clue for exploring the novel spin phenomena. Here we show that the two-component nature is manifested in the Landau levels (LLs) whose degeneracy is lifted by a Coulomb potential. Using spectroscopic-imaging scanning tunneling microscopy, we visualize energy and spatial structures of LLs in a topological insulator Bi2Se3. The observed potential-induced LL splitting and internal structures of Landau orbits are distinct from those in a conventional electron system and are well reproduced by a two-component model Dirac Hamiltonian. Our model further predicts non-trivial energy-dependent spin-magnetization textures in a potential variation. This provides a way to manipulate spins in the topological surface state.
We present magneto-Raman scattering studies of electronic inter Landau level excitations in quasi-neutral graphene samples with different strengths of Coulomb interaction. The band velocity associated with these excitations is found to depend on the dielectric environment, on the index of Landau level involved, and to vary as a function of the magnetic field. This contradicts the single-particle picture of non-interacting massless Dirac electrons, but is accounted for by theory when the effect of electron-electron interaction is taken into account. Raman active, zero-momentum inter Landau level excitations in graphene are sensitive to electron-electron interactions due to the non-applicability of the Kohn theorem in this system, with a clearly non-parabolic dispersion relation.
We construct an action for the composite Dirac fermion consistent with symmetries of electrons projected to the lowest Landau level. First we construct a generalization of the $g=2$ electron that gives a smooth massless limit on any curved background. Using the symmetries of the microscopic electron theory in this massless limit we find a number of constraints on any low-energy effective theory. We find that any low-energy description must couple to a geometry which exhibits nontrivial curvature even on flat space-times. Any composite fermion must have an electric dipole moment proportional and orthogonal to the composite fermions wavevector. We construct the effective action for the composite Dirac fermion and calculate the physical stress tensor and current operators for this theory.
The recent theoretical prediction and experimental realization of topological insulators (TI) has generated intense interest in this new state of quantum matter. The surface states of a three-dimensional (3D) TI such as Bi_2Te_3, Bi_2Se_3 and Sb_2Te_3 consist of a single massless Dirac cones. Crossing of the two surface state branches with opposite spins in the materials is fully protected by the time reversal (TR) symmetry at the Dirac points, which cannot be destroyed by any TR invariant perturbation. Recent advances in thin-film growth have permitted this unique two-dimensional electron system (2DES) to be probed by scanning tunneling microscopy (STM) and spectroscopy (STS). The intriguing TR symmetry protected topological states were revealed in STM experiments where the backscattering induced by non-magnetic impurities was forbidden. Here we report the Landau quantization of the topological surface states in Bi_2Se_3 in magnetic field by using STM/STS. The direct observation of the discrete Landau levels (LLs) strongly supports the 2D nature of the topological states and gives direct proof of the nondegenerate structure of LLs in TI. We demonstrate the linear dispersion of the massless Dirac fermions by the square-root dependence of LLs on magnetic field. The formation of LLs implies the high mobility of the 2DES, which has been predicted to lead to topological magneto-electric effect of the TI.
Inter-Landau-level transitions break particle hole symmetry and will choose either the Pfaffian or the anti-Pfaffian state as the absolute ground state at 5/2 filling of the fractional quantum Hall effect. An approach based on truncating the Hilbert space has favored the anti-Pfaffian. A second approach based on an effective Hamiltonian produced the Pfaffian. In this letter perturbation theory is applied to finite sizes without bias to any specific pseudo-potential component. This method also singles out the anti-Pfaffian. A critical piece of the effective Hamiltonian, which was absent in previous studies, reverts the ground state at 5/2 to the anti-Pfaffian.
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