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Register a new userOut-of-plane nesting driven spin spiral in ultrathin Fe/Cu(001) films
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Epitaxial ultrathin Fe films on fcc Cu(001) exhibit a spin spiral (SS), in contrast to the ferromagnetism of bulk bcc Fe. We study the in-plane and out-of-plane Fermi surfaces (FSs) of the SS in 8 monolayer Fe/Cu(001) films using energy dependent soft x-ray momentum-resolved photoemission spectroscopy. We show that the SS originates in nested regions confined to out-of-plane FSs, which are drastically modified compared to in-plane FSs. From precise reciprocal space maps in successive zones, we obtain the associated real space compressive strain of 1.5+-0.5% along c-axis. An autocorrelation analysis quantifies the incommensurate ordering vector q=(2pi/a)(0,0,~0.86), favoring a SS and consistent with magneto-optic Kerr effect experiments. The results reveal the importance of in-plane and out-of-plane FS mapping for ultrathin films.
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We present a detailed study of the ground-state magnetic structure of ultrathin Fe films on the surface of fcc Ir(001). We use the spin-cluster expansion technique in combination with the relativistic disordered local moment scheme to obtain parameters of spin models and then determine the favored magnetic structure of the system by means of a mean field approach and atomistic spin dynamics simulations. For the case of a single monolayer of Fe we find that layer relaxations very strongly influence the ground-state spin configurations, whereas Dzyaloshinskii-Moriya (DM) interactions and biquadratic couplings also have remarkable effects. To characterize the latter effect we introduce and analyze spin collinearity maps of the system. While for two monolayers of Fe we find a single-q spin spiral as ground state due to DM interactions, for the case of four monolayers the system shows a noncollinear spin structure with nonzero net magnetization. These findings are consistent with experimental measurements indicating ferromagnetic order in films of four monolayers and thicker.
The phase immiscibility and the excellent matching between Ag(001) and Fe(001) unit cells (mismatch 0.8 %) make Fe/Ag growth attractive in the field of low dimensionality magnetic systems. Intermixing could be drastically limited at deposition temperatures as low as 140-150 K. The film structural evolution induced by post-growth annealing presents many interesting aspects involving activated atomic exchange processes and affecting magnetic properties. Previous experiments, of He and low energy ion scattering on films deposited at 150 K, indicated the formation of a segregated Ag layer upon annealing at 550 K. Higher temperatures led to the embedding of Fe into the Ag matrix. In those experiments, information on sub-surface layers was attained by techniques mainly sensitive to the topmost layer. Here, systematic PED measurements, providing chemical selectivity and structural information for a depth of several layers, have been accompanied with a few XRD rod scans, yielding a better sensitivity to the buried interface and to the film long range order. The results of this paper allow a comparison with recent models enlightening the dissolution paths of an ultra thin metal film into a different metal, when both subsurface migration of the deposit and phase separation between substrate and deposit are favoured. The occurrence of a surfactant-like stage, in which a single layer of Ag covers the Fe film is demonstrated for films of 4-6 ML heated at 500-550 K. Evidence of a stage characterized by the formation of two Ag capping layers is also reported. As the annealing temperature was increased beyond 700 K, the surface layers closely resembled the structure of bare Ag(001) with the residual presence of subsurface Fe aggregates.
We present a combined analytical and numerical micromagnetic study of the equilibrium energy, size and shape of anti-skyrmionic magnetic configurations. Anti-skyrmions can be stabilized when the Dzyaloshinskii-Moriya interaction has opposite signs along two orthogonal in-plane directions, breaking the magnetic circular symmetry. We compare the equilibrium energy, size and shape of anti-skyrmions and skyrmions that are stabilized respectively in environments with anisotropic and isotropic Dzyaloshinskii-Moriya interaction, but with the same strength of the magnetic interactions.When the dipolar interactions are neglected the skyrmion and the anti-skyrmion have the same energy, shape and size in their respective environment. However, when dipolar interactions are considered, the energy of the anti-skyrmion is strongly reduced and its equilibrium size increased with respect to the skyrmion. While the skyrmion configuration shows homochiral N{e}el magnetization rotations, anti-skyrmions show partly N{e}el and partly Bloch rotations. The latter do not produce magnetic charges and thus cost less dipolar energy. Both magnetic configurations are stable when the magnetic energies almost cancel each other, which means that a small variation of one parameter can drastically change their configuration, size and energy.
Antiferromagnetic (AFM) domains in ultrathin CoO(001) films are imaged by a wide-field optical microscopy using magneto-optical birefringence effect. The magnetic origin of observed optical contrast is confirmed by the spin orientation manipulation through exchange coupling in Fe/CoO(001) bilayer. The finite size effect of ordering temperature for ultrathin single crystal CoO film is revealed by the thickness and temperature dependent measurement of birefringence contrast. The magneto-optical birefringence effect is found to strongly depend on the photon energy of incident light, and a surprising large polarization rotation angle up to 168.5 mdeg is obtained from a 4.6 nm CoO film with a blue light source, making it possible to further investigate the evolution of AFM domains in AFM ultrathin film under external field.
We investigated head-to-head domain walls in nanostrips of epitaxial $mathrm{Fe}_4mathrm{N}(001)$ thin films, displaying a fourfold magnetic anisotropy. Magnetic force microscopy and micromagnetic simulations show that the domain walls have specific properties, compared to soft magnetic materials. In particular, strips aligned along a hard axis of magnetization are wrapped by partial flux-closure concertina domains below a critical width, while progressively transforming to zigzag walls for wider strips. Transverse walls are favored upon initial application of a magnetic field transverse to the strip, while transformation to a vortex walls is favored upon motion under a longitudinal magnetic field. In all cases the magnetization texture of such fourfold anisotropy domain walls exhibits narrow micro-domain walls, which may give rise to peculiar spin-transfer features.
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