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Register a new userKinetic Magnetism and Orbital Order in Iron Telluride
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Iron telluride (FeTe), a relative of the iron based high temperature superconductors, displays unusual magnetic order and structural transitions. Here we explore the idea that strong correlations may play an important role in these materials. We argue that the unusual orders observed in FeTe can be understood from a picture of correlated local moments with orbital degeneracy, coupled to a small density of itinerant electrons. A component of the structural transition is attributed to orbital, rather than magnetic ordering, introducing a strongly anisotropic character to the system along the diagonal directions of the iron lattice. Double exchange interactions couple the diagonal chains leading to the observed ordering wavevector. The incommensurate order in samples with excess iron arises from electron doping in this scenario. The strong anisotropy of physical properties in the ordered phase should be detectable by transport in single domains. Predictions for ARPES, inelastic neutron scattering and hole/electron doping studies are also made.
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Iron telluride doped lightly with selenium is known to undergo a first order magneto-structural transition before turning superconducting at higher doping. We study the effects of magneto-elastic couplings on this transition using symmetry considerations. We find that the magnetic order parameters are coupled to the uniform monoclinic strain of the unit cell with one iron per cell, as well as to the phonons at high symmetry points of the Brillouin zone. In the magnetic phase the former gives rise to monoclinic distortion while the latter induces dimerization of the ferromagnetic iron chains due to alternate lengthening and shortening of the nearest-neighbour iron-iron bonds. We compare this system with the iron arsenides and propose a microscopic magneto-elastic Hamiltonian which is relevant for all the iron based superconductors. We argue that this describes electron-lattice coupling in a system where electron-electron interaction is crucial.
We study a two-orbital spin model to describe (pi,0) stripe antiferromagnetism in the iron pnictides. The double-spin model has an on-site Hundss coupling and inter-site interactions extending to second neighbors (inter- and intra-orbital) on the square lattice. Using a variational method based on a cluster decomposition, we optimize wave functions with up to 8 cluster sites (up to 2^16 variational parameters). We focus on the anomalously small ordered moments in the stripe state of the pnictides. To account for it, and large variations among different compounds, we show that the second-neighbor cross-orbital exchange constant should be ferromagnetic, which leads to partially hidden stripe order, with a moment that can be varied over a large range by small changes in the coupling constants. In a different parameter region, we confirm the existence of a canted state previously found in spin-wave theory. We also identify several other phases of the model.
Orbital-ordering instability arising due to the intrapocket nesting is investigated for the tight-binding models of pnictides in the presence of orbital-lattice coupling. The incommensurate instabilities with small momentum, which may play an important role in the nematic-ordering transition, vary from model to model besides being more favorable in comparison to the spin-density wave instability in the absence of good interpocket nesting. We also examine the doping dependence of such instabilities. The electron-phonon coupling parameter required to induce them are compared with the first-principle calculations.
Control of emergent magnetic orders in correlated electron materials promises new opportunities for applications in spintronics. For their technological exploitation, it is important to understand the role of surfaces and interfaces to other materials and their impact on the emergent magnetic orders. Here, we demonstrate for iron telluride, the nonsuperconducting parent compound of the iron chalcogenide superconductors, determination and manipulation of the surface magnetic structure by low-temperature spin-polarized scanning tunneling microscopy. Iron telluride exhibits a complex structural and magnetic phase diagram as a function of interstitial iron concentration. Several theories have been put forward to explain the different magnetic orders observed in the phase diagram, which ascribe a dominant role either to interactions mediated by itinerant electrons or to local moment interactions. Through the controlled removal of surface excess iron, we can separate the influence of the excess iron from that of the change in the lattice structure.
In strongly correlated multi-orbital systems, various ordered phases appear. In particular, the orbital order in iron-based superconductors attracts much attention since it is considered to be the origin of the nematic state. In order to clarify the essential condition for realizing orbital orders, we study simple two-orbital ($d_{xz}$, $d_{yz}$) Hubbard model. We find that the orbital order, which corresponds to the nematic order, appears due to the vertex corrections even in the two-orbital model. Thus, $d_{xy}$ orbital is not essential to realize the nematic orbital order. The obtained orbital order depends on the orbital dependence and the topology of fermi surfaces. We also find that another type of orbital order, which is rotated $45^circ$, appears in the heavily hole-doped case.
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