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We present an opto-electrical cooling scheme for polar molecules based on a Sisyphus-type cooling cycle in suitably tailored electric trapping fields. Dissipation is provided by spontaneous vibrational decay in a closed level scheme found in symmetric-top rotors comprising six low-field-seeking rovibrational states. A generic trap design is presented. Suitable molecules are identified with vibrational decay rates on the order of 100Hz. A simulation of the cooling process shows that the molecular temperature can be reduced from 1K to 1mK in approximately 10s. The molecules remain electrically trapped during this time, indicating that the ultracold regime can be reached in an experimentally feasible scheme.
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We present a versatile electric trap for the exploration of a wide range of quantum phenomena in the interaction between polar molecules. The trap combines tunable fields, homogeneous over most of the trap volume, with steep gradient fields at the trap boundary. An initial sample of up to 10^8 CH3F molecules is trapped for as long as 60 seconds, with a 1/e storage time of 12 seconds. Adiabatic cooling down to 120 mK is achieved by slowly expanding the trap volume. The trap combines all ingredients for opto-electrical cooling, which, together with the extraordinarily long storage times, brings field-controlled quantum-mechanical collision and reaction experiments within reach.
We implement a cavity opto-electromechanical system integrating electrical actuation capabilities of nanoelectromechanical devices with ultrasensitive mechanical transduction achieved via intra-cavity optomechanical coupling. Electrical gradient forces as large as 0.40 microN are realized, with simultaneous mechanical transduction sensitivity of 1.5 X 10^-18 m/rtHz representing a three orders of magnitude improvement over any nanoelectromechanical system to date. Opto-electromechanical feedback cooling is demonstrated, exhibiting strong squashing of the in-loop transduction signal. Out-of-loop transduction provides accurate temperature calibration even in the critical paradigm where measurement backaction induces opto-mechanical correlations.
We discuss how the internal structure of ultracold molecules, trapped in the motional ground state of optical tweezers, can be used to implement qudits. We explore the rotational, fine and hyperfine structure of $^{40}$Ca$^{19}$F and $^{87}$Rb$^{133}$Cs, which are examples of molecules with $^2Sigma$ and $^1Sigma$ electronic ground states, respectively. In each case we identify a subset of levels within a single rotational manifold suitable to implement a 4-level qudit. Quantum gates can be implemented using two-photon microwave transitions via levels in a neighboring rotational manifold. We discuss limitations to the usefulness of molecular qudits, arising from off-resonant excitation and decoherence. As an example, we present a protocol for using a molecular qudit of dimension $d=4$ to perform the Deutsch algorithm.
We study the rotational and vibrational heating of diatomic molecules placed near a surface at finite temperature on the basis of macroscopic quantum electrodynamics. The internal molecular evolution is governed by transition rates that depend on both temperature and position. Analytical and numerical methods are used to investigate the heating of several relevant molecules near various surfaces. We determine the critical distances at which the surface itself becomes the dominant source of heating and we investigate the transition between the long-range and short-range behaviour of the heating rates. A simple formula is presented that can be used to estimate the surface-induced heating rates of other molecules of interest. We also consider how the heating depends on the thickness and composition of the surface.
Recently, laser cooling methods have been extended from atoms to molecules. The complex rotational and vibrational energy level structure of molecules makes laser cooling difficult, but these difficulties have been overcome and molecules have now been cooled to a few microkelvin and trapped for several seconds. This opens many possibilities for applications in quantum science and technology, controlled chemistry, and tests of fundamental physics. This article explains how molecules can be decelerated, cooled and trapped using laser light, reviews the progress made in recent years, and outlines some future applications.
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