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Register a new userA Chiral Paramagnetic Skyrmion-like Phase in MnSi
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We present a comprehensive study of chiral fluctuations in the reference helimagnet MnSi by polarized neutron scattering and Neutron Spin Echo spectroscopy, which reveals the existence of a completely left-handed and dynamically disordered phase. This phase may be identified as a spontaneous skyrmion phase: it appears in a limited temperature range just above the helical transition Tc and coexists with the helical phase at Tc.
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A systematic x-ray magnetic circular dichroism study of the paramagnetic phase of ErCo2 has recently allowed to identify the inversion of the net magnetization of the Co net moment with respect to the applied field well above the ferrimagnetic ordering temperature, Tc. The study of small angle neutron scattering measurements has also shown the presence of short range order correlations in the same temperature region. This phenomenon, which we have denoted parimagnetism, may be related with the onset of a Griffiths-like phase in paramagnetic ErCo2. We have measured ac susceptibility on ErCo2 as a function of temperature, applied field, and excitation frequency. Several characteristics shared by systems showing a Griffiths phase are present in ErCo2, namely the formation of ferromagnetic clusters in the disordered phase, the loss of analyticity of the magnetic susceptibility and its extreme sensitivity to an applied magnetic field. The paramagnetic susceptibility allows to establish that the magnetic clusters are only formed by Co moments as well as the intrinsic nature of those Co moments.
We develop a theory of the magnetic field-induced formation of Skyrmion crystal state in chiral magnets in two spatial dimensions, motivated by the recent discovery of the Skyrmionic phase of magnetization in thin film of Fe$_{0.5}$Co$_{0.5}$Si and in the A-phase of MnSi. Ginzburg-Landau functional of the chiral magnet re-written in the CP$^1$ representation is shown to be a convenient framework for the analysis of the Skyrmion states. Phase diagram of the model at zero temperature gives a sequence of ground states, helical spin $rightarrow$ Skyrme crystal $rightarrow$ ferromagnet, as the external field $B$ increases, in good accord with the thin-film experiment. In close analogy with Abrikosovs derivation of the vortex lattice solution in type-II superconductor, the CP$^1$ mean-field equation is solved and shown to reproduce the Skyrmion crystal state.
We present a comprehensive analysis of high resolution neutron scattering data involving Neutron Spin Echo spectroscopy and Spherical Polarimetry which confirm the first order nature of the helical transition and reveal the existence of a new spin liquid skyrmion phase. Similar to the blue phases of liquid crystals this phase appears in a very narrow temperature range between the low temperature helical and the high temperature paramagnetic phases.
Chiral nematic liquid crystals sometimes form blue phases characterized by spirals twisting in different directions. By combining model calculations with neutron-scattering experiments, we show that the magnetic analogue of blue phases does form in the chiral itinerant magnet MnSi in a large part of the phase diagram. The properties of this blue phase explain a number of previously reported puzzling features of MnSi such as partial magnetic order and a two-component specific-heat and thermal-expansion anomaly at the magnetic transition.
We report an experimental study of the emergence of non-trivial topological winding and long-range order across the paramagnetic to skyrmion lattice transition in the transition metal helimagnet MnSi. Combining measurements of the susceptibility with small angle neutron scattering, neutron resonance spin echo spectroscopy and all-electrical microwave spectroscopy, we find evidence of skyrmion textures in the paramagnetic state exceeding $10^3$AA with lifetimes above several 10$^{-9}$s. Our experimental findings establish that the paramagnetic to skyrmion lattice transition in MnSi is well-described by the Landau soft-mode mechanism of weak crystallization, originally proposed in the context of the liquid to crystal transition. As a key aspect of this theoretical model, the modulation-vectors of periodic small amplitude components of the magnetization form triangles that add to zero. In excellent agreement with our experimental findings, these triangles of the modulation-vectors entail the presence of the non-trivial topological winding of skyrmions already in the paramagnetic state of MnSi when approaching the skyrmion lattice transition.
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