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Register a new userWeak crystallization of fluctuating skyrmion textures in MnSi
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Christian Pfleiderer
Publication date
2019
fields
Physics
and research's language is
English
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We report an experimental study of the emergence of non-trivial topological winding and long-range order across the paramagnetic to skyrmion lattice transition in the transition metal helimagnet MnSi. Combining measurements of the susceptibility with small angle neutron scattering, neutron resonance spin echo spectroscopy and all-electrical microwave spectroscopy, we find evidence of skyrmion textures in the paramagnetic state exceeding $10^3$AA with lifetimes above several 10$^{-9}$s. Our experimental findings establish that the paramagnetic to skyrmion lattice transition in MnSi is well-described by the Landau soft-mode mechanism of weak crystallization, originally proposed in the context of the liquid to crystal transition. As a key aspect of this theoretical model, the modulation-vectors of periodic small amplitude components of the magnetization form triangles that add to zero. In excellent agreement with our experimental findings, these triangles of the modulation-vectors entail the presence of the non-trivial topological winding of skyrmions already in the paramagnetic state of MnSi when approaching the skyrmion lattice transition.
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We investigate the anisotropic nature of magnetocrystalline coupling between the crystallographic and skyrmion crystal (SKX) lattices in the chiral magnet MnSi by magnetic field-angle resolved resonant ultrasound spectroscopy. Abrupt changes are observed in the elastic moduli and attenuation when the magnetic field is parallel to the [011] crystallographic direction. These observations are interpreted in a phenomenological Ginzburg-Landau theory that identifies switching of the SKX orientation to be the result of an anisotropic magnetocrystalline coupling potential. Our paper sheds new light on the nature of magnetocrystalline coupling potential relevant to future spintronic applications.
We report high-precision small angle neutron scattering of the orientation of the skyrmion lattice in a spherical sample of MnSi under systematic changes of the magnetic field direction. For all field directions the skyrmion lattice may be accurately described as a triple-$vec{Q}$ state, where the modulus $vert vec{Q} vert$ is constant and the wave vectors enclose rigid angles of $120^{circ}$. Along a great circle across $langle 100rangle$, $langle 110rangle$, and $langle 111rangle$ the normal to the skyrmion-lattice plane varies systematically by $pm3^{circ}$ with respect to the field direction, while the in-plane alignment displays a reorientation by $15^{circ}$ for magnetic field along $langle 100rangle$. Our observations are qualitatively and quantitatively in excellent agreement with an effective potential, that is determined by the symmetries of the tetrahedral point group $T$ and includes contributions up to sixth-order in spin-orbit coupling, providing a full account of the effect of cubic magnetocrystalline anisotropies on the skyrmion lattice in MnSi.
Using small-angle neutron scattering (SANS), we investigate the deformation of the magnetic skyrmion lattice in bulk single-crystalline MnSi under electric current flow. A significant broadening of the skyrmion-lattice-reflection peaks was observed in the SANS pattern for current densities greater than a threshold value j_t ~ 1 MA/m^2 (10^6 A/m^2). We show this peak broadening to originate from a spatially inhomogeneous rotation of the skyrmion lattice, with an inverse rotation sense observed for opposite sample edges aligned with the direction of current flow. The peak broadening (and the corresponding skyrmion lattice rotations) remain finite even after switching off the electric current. These results indicate that skyrmion lattices under current flow experience significant friction near the sample edges, and plastic deformation due to pinning effects, these being important factors that must be considered for the anticipated skyrmion-based applications in chiral magnets at the nanoscale.
Majorana bound states are zero-energy states predicted to emerge in topological superconductors and intense efforts seeking a definitive proof of their observation are still ongoing. A standard route to realize them involves antagonistic orders: a superconductor in proximity to a ferromagnet. Here we show this issue can be resolved using antiferromagnetic rather than ferromagnetic order. We propose to use a chain of antiferromagnetic skyrmions, in an otherwise collinear antiferromagnet, coupled to a bulk conventional superconductor as a novel platform capable of supporting Majorana bound states that are robust against disorder. Crucially, the collinear antiferromagnetic region neither suppresses superconductivity nor induces topological superconductivity, thus allowing for Majorana bound states localized at the ends of the chain. Our model introduces a new class of systems where topological superconductivity can be induced by editing antiferromagnetic textures rather than locally tuning material parameters, opening avenues for the conclusive observation of Majorana bound states.
We present an experimental study of the electronic structure of MnSi. Using X-ray Absorption Spectroscopy, X-ray photoemission and X-ray fluorescence we provide experimental evidence that MnSi has a mixed valence ground state. We show that self consistent LDA supercell calculations cannot replicate the XAS spectra of MnSi, while a good match is achieved within the atomic multiplet theory assuming a mixed valence ground state. We discuss the role of the electron-electron interactions in this compound and estimate that the valence fluctuations are suppressed by a factor of 2.5, which means that the Coulomb repulsion is not negligible.
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