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Dirac Fermions in Graphite: the State of Art

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 Added by Igor Luk'yanchuk A
 Publication date 2009
  fields Physics
and research's language is English




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Macroscopic concentration of massless charge carriers with linear conic spectrum - Dirac Fermions (DF) - was shown in 2004 to exist in highly oriented pyrolytic graphite (HOPG) and governs its electronic properties. These carriers can have the same nature as DF observed in graphite monolayer(graphene) and let to view HOPG as superposition of 2D carbon layers, almost independent electronically. We overview here the recent experimental evidences of 2D DF in graphite and their similarity with carriers in graphene.



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We report on far infrared magneto-transmission measurements on a thin graphite sample prepared by exfoliation of highly oriented pyrolytic graphite. In magnetic field, absorption lines exhibiting a blue-shift proportional to sqrtB are observed. This is a fingerprint for massless Dirac holes at the H point in bulk graphite. The Fermi velocity is found to be c*=1.02x10^6 m/s and the pseudogap at the H point is estimated to be below 10 meV. Although the holes behave to a first approximation as a strictly 2D gas of Dirac fermions, the full 3D band structure has to be taken into account to explain all the observed spectral features.
The recent theoretical prediction and experimental realization of topological insulators (TI) has generated intense interest in this new state of quantum matter. The surface states of a three-dimensional (3D) TI such as Bi_2Te_3, Bi_2Se_3 and Sb_2Te_3 consist of a single massless Dirac cones. Crossing of the two surface state branches with opposite spins in the materials is fully protected by the time reversal (TR) symmetry at the Dirac points, which cannot be destroyed by any TR invariant perturbation. Recent advances in thin-film growth have permitted this unique two-dimensional electron system (2DES) to be probed by scanning tunneling microscopy (STM) and spectroscopy (STS). The intriguing TR symmetry protected topological states were revealed in STM experiments where the backscattering induced by non-magnetic impurities was forbidden. Here we report the Landau quantization of the topological surface states in Bi_2Se_3 in magnetic field by using STM/STS. The direct observation of the discrete Landau levels (LLs) strongly supports the 2D nature of the topological states and gives direct proof of the nondegenerate structure of LLs in TI. We demonstrate the linear dispersion of the massless Dirac fermions by the square-root dependence of LLs on magnetic field. The formation of LLs implies the high mobility of the 2DES, which has been predicted to lead to topological magneto-electric effect of the TI.
We construct an action for the composite Dirac fermion consistent with symmetries of electrons projected to the lowest Landau level. First we construct a generalization of the $g=2$ electron that gives a smooth massless limit on any curved background. Using the symmetries of the microscopic electron theory in this massless limit we find a number of constraints on any low-energy effective theory. We find that any low-energy description must couple to a geometry which exhibits nontrivial curvature even on flat space-times. Any composite fermion must have an electric dipole moment proportional and orthogonal to the composite fermions wavevector. We construct the effective action for the composite Dirac fermion and calculate the physical stress tensor and current operators for this theory.
Pulsed magnetic fields of up to 55T are used to investigate the transport properties of the topological insulator Bi_2Se_3 in the extreme quantum limit. For samples with a bulk carrier density of n = 2.9times10^16cm^-3, the lowest Landau level of the bulk 3D Fermi surface is reached by a field of 4T. For fields well beyond this limit, Shubnikov-de Haas oscillations arising from quantization of the 2D surface state are observed, with the u =1 Landau level attained by a field of 35T. These measurements reveal the presence of additional oscillations which occur at fields corresponding to simple rational fractions of the integer Landau indices.
We investigate Dirac fermions on the surface of the topological insulator Bi2Se3 using scanning tunneling spectroscopy. Landau levels (LLs) are observed in the tunneling spectra in a magnetic field. In contrast to LLs of conventional electrons, a field independent LL appears at the Dirac point, which is a hallmark of Dirac fermions. A scaling analysis of LLs based on the Bohr-Sommerfeld quantization condition allowed us to determine the dispersion of the surface band. Near the Fermi energy, fine peaks mixed with LLs appear in the spectra, which may be responsible for the anomalous magneto-fingerprint effect [J. G. Checkelsky et al., Phys. Rev. Lett. 103, 246601 (2009)].
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