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Register a new userVortex studies in superconducting Ba(Fe0.93Co0.07)2As2
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Morten Ring Eskildsen
Publication date
2008
fields
Physics
and research's language is
English
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We present small-angle neutron scattering (SANS) and Bitter decoration studies of the superconducting vortices in Ba(Fe$_{0.93}$Co$_{0.07}$)$_2$As$_2$}. A highly disordered vortex configuration is observed at all measured fields, and is attributed to strong pinning. This conclusion is supported by the absence of a Meissner rim in decoration images obtained close to the sample edge. The field dependence of the magnitude of the SANS scattering vector indicates vortex lattice domains of (distorted) hexagonal symmetry, consistent with the decoration images which show primarily 6-fold coordinated vortex domains. An analysis of the scattered intensity shows that this decreases much more rapidly than expected from estimates of the upper critical field, consistent with the large degree of disorder.
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The London penetration depth, $lambda(T)$, has been measured in several single crystals of Ba(Fe$_{0.93}$Co$_{0.07}$)$_2$As$_2$. Thermodynamic, electromagnetic, and structural characterization measurements confirm that these crystals are of excellent quality. The observed low temperature variation of $lambda(T)$ follows a power-law, $Delta lambda (T) sim T^n$ with $n=2.4 pm 0.1$, indicating the existence of normal quasiparticles down to at least $0.02T_c$. This is in contrast to recent penetration depth measurements on single crystals of NdFeAsO$_{1-x}$F$_x$ and SmFeAsO$_{1-x}$F$_x$, which indicate an anisotropic but nodeless gap. We propose that a more three-dimensional character in the electronic structure of Ba(Fe$_{0.93}$Co$_{0.07}$)$_2$As$_2$ may lead to an anisotropic $s-$wave gap with point nodes that would explain the observed $lambda(T)$.
Inelastic neutron scattering from superconducting (SC) Ba(Fe$_{0.926}$Co$_{0.074}$)$_2$As$_2$ reveals anisotropic and quasi-two-dimensional (2D) magnetic excitations close to textbf{Q}$_{texttt{AFM}}=({1}{2}/{1}{2})$ - the 2D antiferromagnetic (AFM) wave-vector of the parent BaFe$_2$As$_2$ compound. The correlation length anisotropy of these low energy fluctuations is consistent with spin nematic correlations in the $J_1$-$J_2$ model with $J_1/J_2 sim$ 1. The spin resonance at $sim$8.3 meV in the SC state displays the same anisotropy. The anisotropic fluctuations experimentally evolve into two distinct maxima only along the direction transverse to textbf{Q}$_{texttt{AFM}}$ above $sim$80 meV indicating unusual quasi-propagating excitations.
We present neutron diffraction measurements on single crystal samples of non-superconducting Ba(Fe1-xCrx)2As2 as a function of Cr-doping for 0<=x<=0.47. The average SDW moment is independent of concentration for x<=0.2 and decreases rapidly for x>=0.3. For concentrations in excess of 30% chromium, we find a new G-type antiferromagnetic phase which rapidly becomes the dominant magnetic ground state. Strong magnetism is observed for all concentrations measured and competition between these ordered states and superconductivity naturally explains the absence of superconductivity in the Cr-doped materials.
Neutron diffraction and high-resolution x-ray diffraction studies find that, similar to the closely related underdoped Ba(Fe[1-x]Cox)2As2 superconducting compounds, Ba(Fe0.961Rh0.039)2As2 shows strong evidence of competition and coexistence between superconductivity and antiferromagnetic order below the superconducting transition, Tc = 14 K. The transition temperatures for both the magnetic order and orthorhombic distortion are in excellent agreement with those inferred from resistivity measurements, and both order parameters manifest a distinct decrease in magnitude below Tc. These data suggest that the strong interaction between magnetism and superconductivity is a general feature of electron-doped Ba(Fe[1-x]TMx)2As2 superconductors (TM = Transition Metal).
We show that despite the low anisotropy, strong vortex pinning and high irreversibility field Hirr close to the upper critical field Hc2 of Ba(Fe1-xCox)2As2, the critical current density Jgb across [001] tilt grain boundaries (GBs) of thin film Ba(Fe1-xCox)2As2 bicrystals is strongly depressed, similar to high-Tc cuprates. Our results suggest that weak-linked GBs are characteristic of both cuprates and pnictides because of competing orders, low carrier density, and unconventional pairing symmetry.
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