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Register a new userLongitudinal SDW order in a quasi-1D Ising-like quantum antiferromagnet
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From neutron diffraction measurements on a quasi-1D Ising-like Co$^{rm 2+}$ spin compound BaCo$_{rm 2}$V$_{rm 2}$O$_{rm 8}$, we observed an appearance of a novel type of incommensurate ordering in magnetic fields. This ordering is essentially different from the N{ e}el-type ordering, which is expected for the classical system, and is caused by quantum fluctuation inherent in the quantum spin chain. A Tomonaga-Luttinger liquid (TLL) nature characteristic of the gapless quantum 1D system is responsible for the realization of the incommensurate ordering.
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In the effective Ising spin-1/2 antiferromagnetic chain system BaCo$_2$V$_2$O$_8, the magnetic-field influence is highly anisotropic. For magnetic fields along the easy axis $c$, the N{e}el order is strongly suppressed already for low fields and an incommensurate order is entered above 4 T. We present a detailed study of the magnetic phase diagrams for different magnetic field directions, which are derived from magnetization data, high-resolution thermal expansion and magnetostriction measurements as well as from the thermal conductivity. Zero-field thermal expansion data reveal that the magnetic transition is accompanied by an orthorhombic distortion within the $ab$ plane. Under ambient conditions the crystals are heavily twinned, but the domain orientation can be influenced either by applying uniaxial pressure or a magnetic field along the [100] direction. In addition, our data reveal a pronounced in-plane magnetic anisotropy for fields applied within the $ab$ plane. For $H || [110]$, the magnetic field influence on T$_N$ is weak, whereas for magnetic fields applied along [100], T$_N$ vanishes at about 10 T and the zero-field N{e}el order is completely suppressed as is confirmed by neutron diffraction data. The second-order phase transition strongly suggests a quantum critical point being present at $Hsimeq 10$ T parallel [100], where the N{e}el order probably changes to a spin-liquid state.
The very-low-temperature thermal conductivity (kappa) is studied for BaCo_2V_2O_8, a quasi-one-dimensional Ising-like antiferromagnet exhibiting an unusual magnetic-field-induced order-to-disorder transition. The nearly isotropic transport in the longitudinal field indicates that the magnetic excitations scatter phonons rather than conduct heat. The field dependence of kappa shows a sudden drop at sim 4 T, where the system unndergoes the transition from the Neel order to the incommensurate state. Another dip at lower field of sim 3 T indicates an unknown magnetic transition, which is likely due to the spin-flop transition. Moreover, the kappa(H) in the transverse field shows a very deep valley-like feature, which moves slightly to higher field and becomes sharper upon lowering the temperature. This indicates a magnetic transition induced by the transverse field, which however is not predicted by the present theories for this low-dimensional spin system.
We report on magnetic resonance studies within the magnetically ordered phase of the quasi-1D antiferromagnet LiCuVO_4. Our studies reveal a spin reorientational transition at a magnetic field H_c1 ~ 25 kOe applied within the crystallographical (ab)-plane in addition to the recently observed one at H_c2 ~75 kOe [ M.G. Banks et al., cond-mat/0608554 (2006)]. Spectra of the antiferromagnetic resonance (AFMR) along low-frequency branches can be described in the frame of a macroscopic theory of exchange-rigid planar magnetic structures. These data allow to obtain the anisotropy of the exchange interaction together with a constant of the uniaxial anisotropy. Spectra of 7Li nuclear magnetic resonance (NMR) show that, within the magnetically ordered phase of LiCuVO_4 in the low-field range H < H_c1, a planar spiral spin structure is realized with the spins lying in the (ab)-plane in agreement with neutron scattering studies of B.J. Gibson et al. [Physica B Vol. 350, 253 (2004)]. Based on NMR spectra simulations, the transition at H_c1 can well be described as a spin-flop transition, where the spin plane of the magnetically ordered structure rotates to be perpendicular to the direction of the applied magnetic field. For H > H_c2 ~ 75 kOe, our NMR spectra simulations show that the magnetically ordered structure exhibits a modulation of the spin projections along the direction of the applied magnetic field H.
It is shown that the mechanism of order out of disorder is at work in the antisymmetric pyrochlore antiferromagnet. Quantum as well as thermal fluctuations break the continuous degeneracy of the classical ground state manifold and reduce its symmetry to $mathbb{Z}_3 times mathbb{Z}_2$. The role of anisotropic symmetric exchange is also investigated and we conclude that this discrete like ordering is robust with respect to these second order like interactions. The antisymmetric pyrochlore antiferromagnet is therefore expected to order at low temperatures, whatever the symmetry type of its interactions, in both the classical and semi classical limits.
Electron spin resonance experiments in the quasi-1D S=1/2 antiferromagnet K$_2$CuSO$_4$Cl$_2$ reveal opening of a gap in absence of magnetic ordering, as well as an anisotropic shift of the resonance magnetic field. These features of magnetic excitation spectrum are explained by a crossover between a gapped spinon-type doublet ESR formed in a 1D antiferromagnet with uniform Dzyaloshinskii-Moriya interaction and a Larmor-type resonance of a quasi-1D Heisenberg system
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