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Register a new userCarrier-envelope phase measurement from half-cycle high harmonics
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We present a method to distinguish the high harmonics generated in individual half-cycle of the driving laser pulse by mixing a weak ultraviolet pulse, enabling one to observe the cutoff of each half-cycle harmonic. We show that the detail information of the driving laser pulse, including the laser intensity, pulse duration and carrier-envelope phase, can be {it in situ} retrieved from the harmonic spectrogram. In addition, our results show that this method also distinguishes the half-cycle high harmonics for a pulse longer than 10 fs, suggesting a potential to extend the CEP measurement to the multi-cycle regime.
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We report on tunnel ionization of Xe by 2-cycle, intense, infrared laser pulses and its dependence on carrier-envelope-phase (CEP). At low values of optical field ($E$), the ionization yield is maximum for cos-like pulses with the dependence becoming stronger for higher charge states. At higher $E$-values, the CEP dependence either washes out or flips. A simple phenomenological model is developed that predicts and confirms the observed results. CEP effects are seen to persist for 8-cycle pulses. Unexpectedly, electron rescattering plays an unimportant role in the observed CEP dependence. Our results provide fresh perspectives in ultrafast, strong-field ionization dynamics of multi-electron systems that lie at the core of attosecond science.
We present a joint experimental-theoretical study on the effect of the carrier-envelope phase (CEP) of a few-cycle pulse on the atomic excitation process. We focus on the excitation rates of argon as a function of CEP in the intensity range from 50-300 TW/cm$^2$, which covers the transition between the multiphoton and tunneling regimes. Through numerical simulations based on solving the time-dependent Schr{o}dinger equation (TDSE), we show that the resulting bound-state population is highly sensitive to both the intensity and the CEP. Because the intensity varies over the interaction region, the CEP effect is considerably reduced in the experiment. Nevertheless, the data clearly agree with the theoretical prediction, and the results encourage the use of precisely tailored laser fields to coherently control the strong-field excitation process. We find a markedly different behavior for the CEP-dependent bound-state population at low and high intensities with a clear boundary, which we attribute to the transition from the multiphoton to the tunneling regime.
Two- and multi-dimensional spectroscopy is used in physics and chemistry to obtain structural and dynamical information that would otherwise be invisible by the projection into a one-dimensional data set such as a single emission or absorption spectrum. Here, we introduce a qualitatively new two-dimensional spectroscopy method by employing the carrier-envelope phase (CEP). Instead of measuring spectral vs. spectral information, the combined application of spectral interferometry and CEP control allows the measurement of otherwise inseparable temporal events on an attosecond time scale. As a specific example, we apply this general method to the case of attosecond pulse train generation, where it allows to separate contributions of three different sub-cycle electron quantum paths within one and the same laser pulse, resulting in a better physical understanding and quantification of the transition region between cutoff and plateau harmonics. The CEP-dependent separation in time between two full-cycle spaced attosecond pulses was determined to modulate by (54 +/- 16) attoseconds.
We theoretically study the carrier-envelope phase dependent inversion generated in a two-level system by excitation with a few-cycle pulse. Based on the invariance of the inversion under time reversal of the exciting field, parameters are introduced to characterize the phase sensitivity of the induced inversion. Linear and nonlinear phase effects are numerically studied for rectangular and sinc-shaped pulses. Furthermore, analytical results are obtained in the limits of weak fields as well as strong dephasing, and by nearly degenerate perturbation theory for sinusoidal excitation. The results show that the phase sensitive inversion in the ideal two-level system is a promising route for constructing carrier-envelope phase detectors.
Driving laser wakefield acceleration with extremely short, near single-cycle laser pulses is crucial to the realisation of an electron source that can operate at kHz-repetition rate while relying on modest laser energy. It is also interesting from a fundamental point of view, as the ponderomotive approximation is no longer valid for such short pulses. Through particle-in-cell simulations, we show how the plasma response becomes asymmetric in the plane of laser polarization, and dependent on the carrier-envelope phase (CEP) of the laser pulse. For the case of self-injection, this in turn strongly affects the initial conditions of injected electrons, causing collective betatron oscillations of the electron beam. As a result, the electron beam pointing, electron energy spectrum and the direction of emitted betatron radiation become CEP-dependent. For injection in a density gradient the effect on beam pointing is reduced and the electron energy spectrum is CEP-independent, as electron injection is mostly longitudinal and mainly determined by the density gradient. Our results highlight the importance of controlling the CEP in this regime for producing stable and reproducible relativistic electron beams and identify how CEP effects may be observed in experiments. In the future, CEP control may become an additional tool to control the energy spectrum or pointing of the accelerated electron beam.
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