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Register a new userRenormalized spin wave excitations in the antiferromagnetic Heisenberg-Kondo model for heavy fermions
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Recent inelastic neutron scattering experiments in CeIn3 and CePd2Si2 single crystals, measured spin wave excitations at low temperatures. These two heavy fermion compounds exhibit antiferromagnetic long-range order, but a strong competition between the Ruderman-Kittel-Kasuya-Yosida(RKKY) interaction and Kondo effect is evidenced by their nearly equal Neel and Kondo temperatures. Our aim is to show how magnons such as measured in the antiferromagnetic phase of these Ce compounds, can be described with a microscopic Heisenberg-Kondo model as introduced by J.R.Iglesias, C.Lacroix and B.Coqblin, used before for studies of the non-magnetic phase. The model includes the correlated Ce-4f electrons hybridized with the conduction band, and we consider competing RKKY (Heisenberg-like J_{H}) and Kondo (J_{K}) antiferromagnetic couplings. Carrying on a series of unitary transformations, we perturbatively derive a second-order effective Hamiltonian which, projected onto the antiferromagnetic electron ground state, describes the spin wave excitations, renormalized by their interaction with correlated itinerant electrons. We numerically study how the different parameters of the model influence the renormalization of the magnons, yielding useful information for the analysis of inelastic neutron scattering experiments in antiferromagnetic heavy fermion compounds. We also compare our results with available experimental data, finding good agreement with the spin wave measurements in cubic CeIn3.
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Recent inelastic neutron scattering experiments in CeIn$_{3}$ and CePd$_{2}$Si$_{2}$ single crystals measured spin wave excitations at low temperatures. These two heavy fermion compounds exhibit antiferromagnetic long-range order, but a strong competition between the Ruderman-Kittel-Kasuya-Yosida(RKKY) interaction and Kondo effect is evidenced by their nearly equal Neel and Kondo temperatures. Our aim is to show how magnons such as measured in the antiferromagnetic phase of these Ce compounds, can be described with a microscopic Heisenberg-Kondo model introduced by J.R.Iglesias, C.Lacroix and B.Coqblin, used before for studies of the non-magnetic phase. The model includes the correlated Ce-$4 f$ electrons hybridized with the conduction band, where we also allow for correlations, and we consider competing RKKY (Heisenberg-like $J_{H} $) and Kondo ($J_{K}$) antiferromagnetic couplings. Carrying on a series of unitary transformations, we perturbatively derive a second-order effective Hamiltonian which, projected onto the antiferromagnetic electron ground state, describes the spin wave excitations, renormalized by their interaction with correlated itinerant electrons. We numerically study how the different parameters of the model influence the renormalization of the magnons, yielding useful information for the analysis of inelastic neutron scattering experiments in antiferromagnetic heavy fermion compounds. We also compare our results with the available experimental data, finding good agreement with the spin wave measurements in cubic CeIn$_3$.
We present a spin-rotation-invariant Green-function theory for the dynamic spin susceptibility in the spin-1/2 antiferromagnetic Heisenberg model on a stacked honeycomb lattice. Employing a generalized mean-field approximation for arbitrary temperatures, the thermodynamic quantities (two-spin correlation functions, internal energy, magnetic susceptibility, staggered magnetization, Neel temperature, correlation length) and the spin-excitation spectrum are calculated by solving a coupled system of self-consistency equations for the correlation functions. The temperature dependence of the magnetic (uniform static) susceptibility is ascribed to antiferromagnetic short-range order. The N{e}el temperature is calculated for arbitrary interlayer couplings. Our results are in a good agreement with numerical computations for finite clusters and with available experimental data on the beta-Cu2V2O2 compound.
7Li NMR measurements were performed in the metallic spinel LiV2O4. The temperature dependencies of the line width, the Knight shift and the spin-lattice relaxation rate were investigated in the temperature range 30 mK < T < 280 K. For temperatures T < 1 K we observe a spin-lattice relaxation rate which slows down exponentially. The NMR results can be explained by a spin-liquid behavior and the opening of a spin gap of the order 0.6 K.
The low-temperature elementary spin excitations in the AFM molecular wheel Fe18 were studied experimentally by inelastic neutron scattering and theoretically by modern numerical methods, such as dynamical density matrix renormalization group or quantum Monte Carlo techniques, and analytical spin-wave theory calculations. Fe18 involves eighteen spin-5/2 Fe(III) ions with a Hilbert space dimension of 10^14, constituting a physical system that is situated in a region between microscopic and macroscopic. The combined experimental and theoretical approach allowed us to characterize and discuss the magnetic properties of Fe18 in great detail. It is demonstrated that physical concepts such as the rotational-band or L&E-band concepts developed for smaller rings are still applicable. In particular, the higher-lying low-temperature elementary spin excitations in Fe18 or AFM wheels in general are of discrete antiferromagnetic spin-wave character.
Spin dynamics is calculated in the ferromagnetic (FM) state of the generalized Kondo lattice model taking into account strong on-site correlations between e_g electrons and antiferromagnetic (AFM) exchange among t_{2g} spins. Our study suggests that competing FM double-exchange and AFM super-exchange interaction lead to a rather nontrivial spin-wave spectrum. While spin excitations have a conventional Dq^2 spectrum in the long-wavelength limit, there is a strong deviation from the spin-wave spectrum of the isotropic Heisenberg model close to the zone boundary. The relevance of our results to the experimental data are discussed.
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