Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userIncoherent mid-infrared charge excitation and the high energy anomaly in the photoemission spectra of cuprates
72
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
On the basis of a semi-phenomenological model, it is argued that the high energy anomaly observed in recent photoemission experiments on cuprates is caused by interaction with an overdamped bosonic mode in the mid-infrared region of the spectrum. Analysis of optical conductivity allows to connect this excitation to the incoherent charge response reported for the majority of high Tc materials and some other perovskites. We show that its large damping is an essential feature responsible for the waterfall dispersion and linewidth of the spectral weight.
rate research
Read More
Angle resolved photoelectron spectroscopic measurements have been performed on an insulating cuprate Ca_2CuO_2Cl_2. High resolution data taken along the Gamma to (pi,pi) cut show an additional dispersive feature that merges with the known dispersion of the lowest binding energy feature, which follows the usual strongly renormalized dispersion of ~0.35 eV. This higher energy part reveals a dispersion that is very close to the unrenormalized band predicted by band theory. A transfer of spectral weight from the low energy feature to the high energy feature is observed as the Gamma point is approached. By comparing with theoretical calculations the high energy feature observed here demonstrates that the incoherent portion of the spectral function has significant structure in momentum space due to the presence of various energy scales.
We used polarization-dependent angle-resolved photoemission spectroscopy (ARPES) to study the high-energy anomaly (HEA) in the dispersion of Nd2-xCexCuO4, (x=0.123). We have found that at particular photon energies the anomalous, waterfalllike dispersion gives way to a broad, continuous band. This suggests that the HEA is a matrix element effect: it arises due to a suppression of the intensity of the broadened quasi-particle band in a narrow momentum range. We confirm this interpretation experimentally, by showing that the HEA appears when the matrix element is suppressed deliberately by changing the light polarization. Calculations of the matrix element using atomic wave functions and simulation of the ARPES intensity with one-step model calculations provide further proof for this scenario. The possibility to detect the full quasi-particle dispersion further allows us to extract the high-energy self-energy function near the center and at the edge of the Brillouin zone.
The anomalous high-energy dispersion of the conductance band in the high-Tc superconductor Pb-Bi2212 has been extensively mapped by angle-resolved photoemission (ARPES) as a function of excitation energy in the range from 34 to 116 eV. Two distinctive types of dispersion behavior are observed around 0.6 eV binding energy, which alternate as a function of photon energy. The continuous transitions observed between the two kinds of behavior near 50, 70, and 90 eV photon energies allow to exclude the possibility that they originate from the interplay between the bonding and antibonding bands. The effects of three-dimensionality can also be excluded as a possible origin of the excitation energy dependence, as the large period of the alterations is inconsistent with the lattice constant in this material. We therefore confirm that the strong photon energy dependence of the high-energy dispersion in cuprates originates mainly from the photoemission matrix element that suppresses the photocurrent in the center of the Brillouin zone.
While charge density wave (CDW) instabilities are ubiquitous to superconducting cuprates, the different ordering wavevectors in various cuprate families have hampered a unified description of the CDW formation mechanism. Here we investigate the temperature dependence of the low energy phonons in the canonical CDW ordered cuprate La$_{1.875}$Ba$_{0.125}$CuO$_{4}$. We discover that the phonon softening wavevector associated with CDW correlations becomes temperature dependent in the high-temperature precursor phase and changes from a wavevector of 0.238 reciprocal space units (r.l.u.) below the ordering transition temperature up to 0.3~r.l.u. at 300~K. This high-temperature behavior shows that 214-type cuprates can host CDW correlations at a similar wavevector to previously reported CDW correlations in non-214-type cuprates such as YBa$_{2}$Cu$_{3}$O$_{6+delta}$. This indicates that cuprate CDWs may arise from the same underlying instability despite their apparently different low temperature ordering wavevectors.
The occupied and the unoccupied electronic structure of CeAg$_2$Ge$_2$ single crystal has been studied using high resolution photoemission and inverse photoemission spectroscopy respectively. High resolution photoemission reveals the clear signature of Ce $4f$ states in the occupied electronic structure which was not observed earlier due to the poor resolution. The coulomb correlation energy in this system has been determined experimentally from the position of the $4f$ states above and below the Fermi level. Theoretically the correlation energy has been determined by using the first principles density functional calculations within the generalized gradient approximations taking into account the strong intra-atomic (on-site) interaction Hubbard $U_{eff}$ term. Although the valence band calculated with different $U_{eff}$ does not show significant difference, but the substantial changes are observed in the conduction band. The estimated value of correlation energy from both the theory and the experiment is $approx$4.2~eV for CeAg$_2$Ge$_2$.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
