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The Gamma Factory (GF) initiative aims at construction of a unique experimental tool exploiting resonant interaction of light with ultra-relativistic partially stripped ions (PSI) stored in circular accelerators at CERN. Resonant excitation of high-energy transitions of the ions is achieved through Doppler-boosting (by twice the Larmor factor; from hundred to several thousand times) of light energy. In order to efficiently excite the ions, and hence generate intense beams of scattered/fluorescent photons, a detailed knowledge of the ions energy structure and dynamics of optical pumping is required. Spectroscopic properties of PSI selected for the GF operation, as well as their optical pumping schemes are investigated. Two regimes of the light-ion interaction are identified, leading to different dynamics of the pumping process. The efficiency of the light-ion interaction as well as the number of photons emitted from a single ion bunch is estimated, both analytically and numerically, for three ions considered for the GF, i.e.~Li-like ${}^{208}_{phantom{0}82}$Pb$^{79+}$, Li-like ${}^{40}_{20}$Ca$^{17+}$, and H-like ${}^{208}_{phantom{0}82}$Pb$^{81+}$.
We demonstrate rotational and vibrational cooling of cesium dimers by optical pumping techniques. We use two laser sources exciting all the populated rovibrational states, except a target state that thus behaves like a dark state where molecules pile
We demonstrate the conversion of cold Cs_{2} molecules initially distributed over several vibrational levels of the lowest triplet state a^{3}Sigma_{u}^{+} into the singlet ground state X^{1}Sigma_{g}^{+}. This conversion is realized by a broadband l
We have recently demonstrated that optical pumping methods combined with photoassociation of ultra-cold atoms can produce ultra-cold and dense samples of molecules in their absolute rovibronic ground state. More generally, both the external and inter
Ionization potentials, excitation energies, transition properties, and hyperfine structure constants of the low-lying $3p^6 3d^{9} ^2D_{5/2}$, $3p^6 3d^{9} ^2D_{3/2}$, $3p^5 3d^{10} ^2P_{3/2}$ and $3p^5 3d^{10} ^2P_{1/2}$ atomic states of the Co-
We present measurements of the hyperfine coefficients and isotope shifts of the Dy I $683.731 $nm transition, using saturated absorption spectroscopy on an atomic beam. A King Plot is drawn resulting in an updated value for the specific mass shift $d