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We report two novel effects in an inhomogeneous ensemble of two-level systems driven by an external field. First, we observe a rigidity of the oscillation frequency: the dominant Rabi oscillation frequency does not change with the frequency of the driving field, in contrast to the well-known law of Rabi frequency increase with growing detuning of the driving field. Second, we observe a time-dependent frequency shift of the ensemble-averaged oscillation. We show that these effects follow from the inhomogeneity of the two-level splitting across the ensemble, allowing for a distribution of local oscillations in which those with high frequencies interfere destructively and decay faster than those with a low frequency, which are the only to survive in the output signal. Hence, coherence emerges from long-lived oscillations in an inhomogeneous ensemble. We analyze the Fourier spectrum of the time-dependent oscillation signal and find a non-trivial spectral structure that is double peaked for certain parameters. We show that the effects observed in alkali vapor are universal and expected in any system with a moderate inhomogeneity driven by an external field.
We investigate the collective scattering of coherent light from a thermal alkali-metal vapor with temperatures ranging from 350 to 450 K, corresponding to average atomic spacings between $0.7 lambda$ and $0.1 lambda$. We develop a theoretical model t
We review methods for coherently controlling Rydberg quantum states of atomic ensembles using Adiabatic Rapid Passage and Stimulated Raman Adiabatic Passage. These methods are commonly used for population inversion in simple two-level and three-level
In analog to counterparts widely used in electronic circuits, all optical non-reciprocal devices are basic building blocks for both classical and quantum optical information processing. Approaching the fundamental limit of such devices, where the pro
We present a combined theoretical and experimental study of solid-state spin decoherence in an electronic spin bath, focusing specifically on ensembles of nitrogen vacancy (NV) color centers in diamond and the associated substitutional nitrogen spin
Using coherent states as initial states, we investigate the quantum dynamics of the Lipkin-Meshkov-Glick (LMG) and Dicke models in the semi-classical limit. They are representative models of bounded systems with one- and two-degrees of freedom, respe