ترغب بنشر مسار تعليمي؟ اضغط هنا

The anomalous magnetic properties of $CaRuO_3$ probed by AC and DC magnetic measurements and by low Ti impurity doping

149   0   0.0 ( 0 )
 نشر من قبل Ivica M. Bradaric
 تاريخ النشر 2017
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

Calcium ruthenate ($CaRuO_3$) is widely believed to be located close to a quantum critical point due to the strong non-Fermi-liquid behavior expressed in the temperature dependence of electronic transport, specific heat, optical conductivity, etc. However, the corresponding anomalous behavior, marking crossover temperature regimes in the magnetic response of $CaRuO_3$, is still lacking. Here we report detailed AC and DC magnetic susceptibility measurements of $CaRuO_3$ and $CaRu_{0.97}Ti_{0.03}O_3$. The AC magnetic susceptibility measurements of the $CaRuO_3$ show a slight dependence on the frequency of AC magnetic field below ~ 40 K, and an additional subtle change of curvature around 12 K. We interpret these results as a critical slowing down of spin fluctuations towards T=0 K. We confirm these observations by magnetic measurements of $CaRu_{0.97}Ti_{0.03}O_3$, which show a pronounced magnetic response corresponding to the above temperatures.

قيم البحث

اقرأ أيضاً

We have studied the magnetic torque in uranium monosulfide (US) single crystals to explore the magnetic anisotropy in this material. Uranium monosulfide crystallizes in cubic, NaCl-type of crystal structure and exhibits the largest magneto-crystallin e anisotropy observed in cubic systems. By performing detailed torque measurements we observe a strongly anisotropic behavior in the paramagnetic phase due to crystal defects and quadrupolar pair interactions. Our studies also confirm the presence of a large anisotropy in the ferromagnetic state of the US system with the <100>, <111>, and <110> directions being hard, easy, and intermediate axis, respectively. Furthermore, the anisotropy in the paramagnetic phase shows similar characteristics to the anisotropy observed in the ferromagnetic phase, as characterized by second and fourth rank susceptibility terms. The similarity of the anisotropic behaviors in paramagnetic and ferromagnetic phases is the consequence of strong magneto-elastic properties in this system, which possibly lead to the rhombohedral structural distortion, not only in the ferromagnetic phase but also in the paramagnetic phase (induced by applied magnetic fiield).
65 - S. Kundu , T. K. Nath 2010
We have thoroughly investigated the entire magnetic states of under doped ferromagnetic insulating manganite Nd0.8Sr0.2MnO3 through temperature dependent linear and non linear complex ac magnetic susceptibility measurements. This ferromagnetic insula ting manganite is found to have frequency independent ferromagnetic to paramagnetic transition temperature at around 140 K. At around 90 K (approx T_f) the sample shows a second frequency dependent re - entrant magnetic transition as explored through complex ac susceptibility measurements. Non linear ac susceptibility measurements (higher harmonics of ac susceptibility) have also been performed (with and without the superposition of a dc magnetic field) to further investigate the origin of this frequency dependence (dynamic behavior at this re-entrant magnetic transition). Divergence of 3rd order susceptibility in the limit of zero exciting field indicates a spin glass like freezing phenomena. However, large value of spin relaxation time (?0= 10-8 s) and small value of coercivity (~22 Oe) obtained at low temperature (below T_f) from critical slowing down model and dc magnetic measurements, respectively, are in contrast with what generally observed in a canonical spin glass (?0 = 10-12 - 10-14 s and very large value of coercivity below freezing temperature). We have attributed our observation to the formation of finite size ferromagnetic clusters which are formed as consequence of intrinsic separation and undergo cluster glass like freezing below certain temperature in this under doped manganite. The results are supported by the electronic - and magneto - transport data.
224 - C. R. Rotundu , B. Andraka 2004
Specific heat for single crystalline samples of Ce1-xLaxOs4Sb12 at zero-field and magnetic fields to 14 T is reported. Our results confirm enhanced value of the electronic specific heat coefficient in the paramagnetic state. They provide arguments fo r the intrinsic origin of the 1.1 K anomaly. This transition leads to opening of the gap at the Fermi surface. This low temperature state of CeOs4Sb12 is extremely sensitive to chemical impurities. 2% of La substituted for Ce suppresses the transition and reduces the electronic specific heat coefficient. The magnetic field response of the specific heat is also anomalous.
Ultrasound velocity measurements of cubic spinel GeCo$_2$O$_4$ in single crystal were performed for the investigation of shear and compression moduli. The shear moduli in the paramagnetic state reveal an absence of Jahn-Teller activity despite the pr esence of orbital degeneracy in the Co$^{2+}$ ions. Such a Jahn-Teller inactivity indicates that the intersite orbital-orbital interaction is much stronger than the Jahn-Teller coupling. The compression moduli in the paramagnetic state near the N$acute{e}$el temperature $T_N$ reveal that the most relevant exchange path for the antiferromagnetic transition lies in the [111] direction. This exchange-path anisotropy is consistent with the antiferromagnetic structure with the wave vector $q parallel$ [111], suggesting the presence of bond frustration due to competition among a direct ferromagnetic and several distant-neighbors antiferromagnetic interactions. In the JT-inactive condition, the bond frustration can be induced by geometrical orbital frustration of $t_{2g}$-$t_{2g}$ interaction between the Co$^{2+}$ ions which can be realized in the pyrochlore lattice of the high spin Co$^{2+}$ with $t_{2g}$-orbital degeneracy. In GeCo$_2$O$_4$, the tetragonal elongation below $T_N$ releases the orbital frustration by quenching the orbital degeneracy.
429 - Z. Y. Zhao , X. M. Wang , C. Fan 2010
The low-temperature thermal conductivity (kappa) of GdFeO_3 single crystals is found to be strongly dependent on magnetic field. The low-field kappa (H) curves show two dips for H parallel a and only one dip for H parallel c, with the characteristic fields having good correspondence with the spin-flop and the spin-polarization transitions. A remarkable phenomenon is that the subKelvin thermal conductivity shows hysteretic behaviors on the history of applying magnetic field, that is, the kappa(H) isotherms measured with field increasing are larger than those with field decreasing. Intriguingly, the broad region of magnetic field (sim 0--3 T) showing the irreversibility of heat transport coincides with that presenting the ferroelectricity. It is discussed that the irreversible kappa(H) behaviors are due to the phonon scattering by ferroelectric domain walls. This result shows an experimental feature that points to the capability of controlling the ferroelectric domain structures by magnetic field in multiferroic materials.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا