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Photothermal heterodyne imaging of individual nonfluorescent nanoclusters and nanocrystals

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 نشر من قبل Laurent Cognet
 تاريخ النشر 2007
  مجال البحث فيزياء
والبحث باللغة English
 تأليف Stephane Berciaud




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We introduce a new, highly sensitive, and simple heterodyne optical method for imaging individual nonfluorescent nanoclusters and nanocrystals. A 2 order of magnitude improvement of the signal is achieved compared to previous methods. This allows for the unprecedented detection of individual small absorptive objects such as metallic clusters (of 67 atoms) or nonluminescent semiconductor nanocrystals. The measured signals are in agreement with a calculation based on the scattering field theory from a photothermal-induced modulated index of refraction profile around the nanoparticle.

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