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We report experimental observations of the convection-driven fingering instability of an iodate-arsenous acid chemical reaction front. The front propagated upward in a vertical slab; the thickness of the slab was varied to control the degree of instability. We observed the onset and subsequent nonlinear evolution of the fingers, which were made visible by a {it p}H indicator. We measured the spacing of the fingers during their initial stages and compared this to the wavelength of the fastest growing linear mode predicted by the stability analysis of Huang {it et. al.} [{it Phys. Rev. E}, {bf 48}, 4378 (1993), and unpublished]. We find agreement with the thickness dependence predicted by the theory.
The extent and the morphology of ice forming in a differentially heated cavity filled with water is studied by means of experiments and numerical simulations. We show that the main mechanism responsible for the ice shaping is the existence of a cold
Large molecules such as proteins and nucleic acids are crucial for life, yet their primordial origin remains a major puzzle. The production of large molecules, as we know it today, requires good catalysts, and the only good catalysts we know that can
Starting from our recent chemical master equation derivation of the model of an autocatalytic reaction-diffusion chemical system with reactions $U+2V {stackrel {lambda_0}{rightarrow}}~ 3 V;$ and $V {stackrel {mu}{rightarrow}}~P$, $U {stackrel { u}{ri
The emergence of self-sustaining autocatalytic networks in chemical reaction systems has been studied as a possible mechanism for modelling how living systems first arose. It has been known for several decades that such networks will form within syst
We revisit the problem of pinning a reaction-diffusion front by a defect, in particular by a reaction-free region. Using collective variables for the front and numerical simulations, we compare the behaviors of a bistable and monostable front. A bist