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We investigate a novel hybrid system composed of an ensemble of room temperature rare-earth ions embedded in a bulk crystal, intrinsically coupled to internal strain via the surrounding crystal field. We evidence the generation of a mechanical response under resonant light excitation. Thanks to an ultra-sensitive time- and space-resolved photodeflection setup, we interpret this motion as the sum of two resonant optomechanical backaction processes: a conservative, piezoscopic process induced by the optical excitation of a well-defined electronic configuration, and a dissipative, non-radiative photothermal process related to the phonons generated throughout the atomic population relaxation. Parasitic heating processes, namely off-resonant dissipative contributions, are absent. This work demonstrates an unprecedented level of control of the conservative and dissipative relative parts of the optomechanical backaction, confirming the potential of rare-earth-based systems as promising hybrid mechanical systems.
Nano-structuring impurity-doped crystals affects the phonon density of states and thereby modifies the atomic dynamics induced by interaction with phonons. We propose the use of nano-structured materials in the form of powders or phononic bandgap cry
We have obtained a low optical inhomogeneous linewidth of 25 MHz in the stoichiometric rare earth crystal EuCl3 .6H2 O by isotopically purifying the crystal in 35 Cl. With this linewidth, an important limit for stoichiometric rare earth crystals is s
The perovskite rare-earth titanates are model Mott insulators with magnetic ground states that are sensitive to structural distortions. These distortions couple strongly to the orbital degrees of freedom and, in principle, it should be possible to tu
Quantum light-matter interfaces (QLMIs) connecting stationary qubits to photons will enable optical networks for quantum communications, precise global time keeping, photon switching, and studies of fundamental physics. Rare-earth-ion (REI) doped cry
Electro-optical control of on-chip photonic devices is an essential tool for efficient integrated photonics. Lithium niobate on insulator (LNOI) is an emerging platform for on-chip photonics due to its large electro-optic coefficient and high nonline