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تسجيل مستخدم جديدUltrafast Measurements of the Interfacial Spin Seebeck Effect in Au and Rare-Earth Iron Garnet Bilayers
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We investigate picosecond spin-currents across Au/iron-garnet interfaces in response to ultrafast laser heating of the electrons in the Au film. In the picoseconds after optical heating, interfacial spin currents occur due to an interfacial temperature difference between electrons in the metal and magnons in the insulator. We report measurements of this interfacial longitudinal spin Seebeck effect between Au and rare-earth iron-garnet insulators, i.e. RE$_3$ Fe$_5$O$_{12}$, where RE is Y, Eu, Tb, Tm. We use time domain thermoreflectance (TDTR) measurements to characterize the thermal response of the bilayer to ultrafast optical heating. We use time-resolved magneto-optic Kerr effect (TR-MOKE) measurements of the Au layer to measure the time-evolution of spin accumulation in the Au film. We observe a spin Seebeck effect between Au/TmIG that is three times larger than for an Au/YIG bilayer. The interfacial thermal conductance between electrons in the Au and magnons in the TmIG layer is ~ 3 $frac{MW}{m^2 K}$.
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For longitudinal spin Seebeck effect (LSSE) devices, a multilayer structure comprising ferromagnetic and nonmagnetic layers is expected to improve their thermoelectric power. In this study, we developed the fabrication method for alternately stacked
yttrium-iron-garnet (YIG)/Pt multilayer films on a gadolinium gallium garnet (GGG) (110) substrate, GGG/[YIG(49 nm)/Pt(4 nm)]$_n$ ($n =$ 1 - 5) based on room-temperature sputtering and $ex$-$situ$ post-annealing method and we evaluated their structural and LSSE properties. The fabricated [YIG/Pt]$_n$ samples show flat YIG/Pt interfaces and almost identical saturation magnetization $M_{rm s}$, although they contain polycrystalline YIG layers on Pt layers as well as single-crystalline YIG layers on GGG. In the samples, we observed clear LSSE signals and found that the LSSE thermoelectric power factor (PF) increases monotonically with increasing $n$; the PF of the [YIG/Pt]$_5$ sample is enhanced by a factor of $sim 28$ compared to that of [YIG/Pt]$_1$. This work may provide a guideline for developing future multilayerbased LSSE devices.
The longitudinal spin Seebeck effect refers to the generation of a spin current when heat flows across a normal metal/magnetic insulator interface. Until recently, most explanations of the spin Seebeck effect use the interfacial temperature differenc
e as the conversion mechanism between heat and spin fluxes. However, recent theoretical and experimental works claim that a magnon spin current is generated in the bulk of a magnetic insulator even in the absence of an interface. This is the so-called intrinsic spin Seebeck effect. Here, by utilizing a non-local spin Seebeck geometry, we provide additional evidence that the total magnon spin current in the ferrimagnetic insulator yttrium iron garnet (YIG) actually contains two distinct terms: one proportional to the gradient in the magnon chemical potential (pure magnon spin diffusion), and a second proportional to the gradient in magnon temperature ($ abla T_m$). We observe two characteristic decay lengths for magnon spin currents in YIG with distinct temperature dependences: a temperature independent decay length of ~ 10 ${mu}$m consistent with earlier measurements of pure ($ abla T_m = 0$) magnon spin diffusion, and a longer decay length ranging from about 20 ${mu}$m around 250 K and exceeding 80 ${mu}$m at 10 K. The coupled spin-heat transport processes are modeled using a finite element method revealing that the longer range magnon spin current is attributable to the intrinsic spin Seebeck effect ($ abla T_m eq 0$), whose length scale increases at lower temperatures in agreement with our experimental data.
Spin waves can probe the Dzyaloshinskii-Moriya interaction (DMI) which gives rise to topological spin textures, such as skyrmions. However, the DMI has not yet been reported in yttrium iron garnet (YIG) with arguably the lowest damping for spin waves
. In this work, we experimentally evidence the interfacial DMI in a 7~nm-thick YIG film by measuring the nonreciprocal spin wave propagation in terms of frequency, amplitude and most importantly group velocities using all electrical spin-wave spectroscopy. The velocities of propagating spin waves show chirality among three vectors, i.e. the film normal direction, applied field and spin-wave wavevector. By measuring the asymmetric group velocities, we extract a DMI constant of 16~$mu$J/m$^{2}$ which we independently confirm by Brillouin light scattering. Thickness-dependent measurements reveal that the DMI originates from the oxide interface between the YIG and garnet substrate. The interfacial DMI discovered in the ultrathin YIG films is of key importance for functional chiral magnonics as ultra-low spin-wave damping can be achieved.
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