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The electric dipole moment of the electron (eEDM) can be measured with high precision using heavy polar molecules. In this paper, we report on a series of new techniques that have improved the statistical sensitivity of the YbF eEDM experiment. We increase the number of molecules participating in the experiment by an order of magnitude using a carefully designed optical pumping scheme. We also increase the detection efficiency of these molecules by another order of magnitude using an optical cycling scheme. In addition, we show how to destabilise dark states and reduce backgrounds that otherwise limit the efficiency of these techniques. Together, these improvements allow us to demonstrate a statistical sensitivity of $1.8 times 10^{-28}$ e cm after one day of measurement, which is 1.2 times the shot-noise limit. The techniques presented here are applicable to other high-precision measurements using molecules.
We describe the first precision measurement of the electrons electric dipole moment (eEDM, $d_e$) using trapped molecular ions, demonstrating the application of spin interrogation times over 700 ms to achieve high sensitivity and stringent rejection
We demonstrate one-dimensional sub-Doppler laser cooling of a beam of YbF molecules to 100 $mu$K. This is a key step towards a measurement of the electrons electric dipole moment using ultracold molecules. We compare the effectiveness of magnetically
We report on a new measurement of the CP-violating permanent Electric Dipole Moment (EDM) of the neutral $^{129}$Xe atom. Our experimental approach is based on the detection of the free precession of co-located nuclear spin-polarized $^3$He and $^{12
We propose an experimental search for an axion-induced oscillating electric dipole moment (OEDM) for electrons using state-of-the-art alkali vapor-cell atomic magnetometers. The axion is a hypothesized new fundamental particle which can resolve the s
We describe a new technique to measure the EDM of $^{129}$Xe with $^3$He comagnetometry. Both species are polarized using spin-exchange optical pumping, transferred to a measurement cell, and transported into a magnetically shielded room, where SQUID