ترغب بنشر مسار تعليمي؟ اضغط هنا

Realisation of Symmetry Enforced Two-Dimensional Dirac Fermions in Nonsymmorphic $alpha$-Bismuthene

118   0   0.0 ( 0 )
 نشر من قبل Guang Bian
 تاريخ النشر 2019
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

Two-dimensional (2D) Dirac-like electron gases have attracted tremendous research interest ever since the discovery of free-standing graphene. The linear energy dispersion and non-trivial Berry phase play the pivotal role in the remarkable electronic, optical, mechanical and chemical properties of 2D Dirac materials. The known 2D Dirac materials are gapless only within certain approximations, for example, in the absence of SOC. Here we report a route to establishing robust Dirac cones in 2D materials with nonsymmorphic crystal lattice. The nonsymmorphic symmetry enforces Dirac-like band dispersions around certain high-symmetry momenta in the presence of SOC. Through $mu$-ARPES measurements we observe Dirac-like band dispersions in $alpha$-bismuthene. The nonsymmorphic lattice symmetry is confirmed by $mu$-LEED and STM. Our first-principles simulations and theoretical topological analysis demonstrate the correspondence between nonsymmorphic symmetry and Dirac states. This mechanism can be straightforwardly generalized to other nonsymmorphic materials. The results open the door for the search of symmetry enforced Dirac fermions in the vast uncharted world of nonsymmorphic 2D materials.

قيم البحث

اقرأ أيضاً

Two-dimensional Dirac semimetals have attracted much attention because of their linear energy dispersion and non-trivial Berry phase. Graphene-like 2D Dirac materials are gapless only within certain approximations, e.g., if spin-orbit coupling (SOC) is neglected. It has recently been reported that materials with nonsymmorphic crystal lattice possess symmetry-enforced Dirac-like band dispersion around certain high-symmetry momenta even in the presence of SOC. Here we calculate the optical absorption coefficient of nonsymmorphic semimetals, such as $alpha$-bismuthene, which hosts two anisotropic Dirac cones with different Fermi velocities along $x$ and $y$ directions.We find that the optical absorption coefficient depends strongly on the anisotropy factor and the photon polarization. When a magnetic field is applied perpendicular to the plane of the material, the absorption coefficient also depends on an internal parameter we termed the mixing angle of the band structure. We further find that an in-plane magnetic field, while leaving the system gapless, can induce a Van-Hove singularity in the joint density of states: this causes a significant enhancement of the optical absorption at the frequency of the singularity for one direction of polarization but not for the orthogonal one, making the optical properties even more strongly dependent on polarization. Due to the anisotropy present in our model, the Dirac cones at two high-symmetry momenta in the Brillouin zone contribute very differently to the optical absorbance. Consequently, it might be possible to preferentially populate one valley or the other by varying photon polarization and frequency. These results suggest that nonsymmorphic 2D Dirac semimetals are excellent candidate materials for tunable magneto-optic devices.
Recent developments in the relationship between bulk topology and surface crystal symmetry have led to the discovery of materials whose gapless surface states are protected by crystal symmetries. In fact, there exists only a very limited set of possi ble surface crystal symmetries, captured by the 17 wallpaper groups. We show that a consideration of symmetry-allowed band degeneracies in the wallpaper groups can be used to understand previous topological crystalline insulators, as well as to predict new examples. In particular, the two wallpaper groups with multiple glide lines, $pgg$ and $p4g$, allow for a new topological insulating phase, whose surface spectrum consists of only a single, fourfold-degenerate, true Dirac fermion. Like the surface state of a conventional topological insulator, the surface Dirac fermion in this nonsymmorphic Dirac insulator provides a theoretical exception to a fermion doubling theorem. Unlike the surface state of a conventional topological insulator, it can be gapped into topologically distinct surface regions while keeping time-reversal symmetry, allowing for networks of topological surface quantum spin Hall domain walls. We report the theoretical discovery of new topological crystalline phases in the A$_2$B$_3$ family of materials in SG 127, finding that Sr$_2$Pb$_3$ hosts this new topological surface Dirac fermion. Furthermore, (100)-strained Au$_2$Y$_3$ and Hg$_2$Sr$_3$ host related topological surface hourglass fermions. We also report the presence of this new topological hourglass phase in Ba$_5$In$_2$Sb$_6$ in SG 55. For orthorhombic space groups with two glides, we catalog all possible bulk topological phases by a consideration of the allowed non-abelian Wilson loop connectivities, and we develop topological invariants for these systems. Finally, we show how in a particular limit, these crystalline phases reduce to copies of the SSH model.
Dirac semimetals, the materials featured with discrete linearly crossing points (called Dirac points) between four bands, are critical states of topologically distinct phases. Such gapless topological states have been accomplished by a band-inversion mechanism, in which the Dirac points can be annihilated pairwise by perturbations without changing the symmetry of the system. Here, we report an experimental observation of Dirac points that are enforced completely by the crystal symmetry, using a nonsymmorphic three-dimensional phononic crystal. Intriguingly, our Dirac phononic crystal hosts four spiral topological surface states, in which the surface states of opposite helicities intersect gaplessly along certain momentum lines, as confirmed by our further surface measurements. The novel Dirac system may release new opportunities for studying the elusive (pseudo)relativistic physics, and also offer a unique prototype platform for acoustic applications.
Filling-enforced Dirac semimetals, or those required at specific fillings by the combination of crystalline and time-reversal symmetries, have been proposed and discovered in numerous materials. However, Dirac points in these materials are not genera lly robust against breaking or modifying time-reversal symmetry. We present a new class of two-dimensional Dirac semimetal protected by the combination of crystal symmetries and a special, antiferromagnetic time-reversal symmetry. Systems in this class of magnetic layer groups, while having broken time-reversal symmetry, still respect the operation of time-reversal followed by a half-lattice translation. In contrast to 2D time-reversal-symmetric Dirac semimetal phases, this magnetic Dirac phase is capable of hosting just a single isolated Dirac point at the Fermi level, and that Dirac point can be stabilized solely by symmorphic crystal symmetries. We find that this Dirac point represents a new quantum critical point, and lives at the boundary between Chern insulating, antiferromagnetic topological crystalline insulating, and trivial insulating phases. We present density functional theoretic calculations which demonstrate the presence of this 2D magnetic Dirac semimetallic phase in FeSe monolayers and discuss the implications for engineering quantum phase transitions in these materials.
Realizing stable two-dimensional (2D) Dirac points against spin-orbit coupling (SOC) has attracted much attention because it provides a platform to study the unique transport properties. In previous work, Young and Kane [Phys. Rev. Lett. textbf{115}, 126803 (2015)] proposed stable 2D Dirac points with SOC, in which the Berry curvature and edge states vanish due to the coexistence of inversion and time-reversal symmetries. Herein, using the tight-binding model and k$cdot$p effective Hamiltonian, we present that 2D Dirac points can survive in the presence of SOC without inversion symmetry. Such 2D Dirac semimetals possess nonzero Berry curvature near the crossing nodes, and two edge states are terminated at one pair of Dirac points. In addition, according to symmetry arguments and high-throughput first-principles calculations, we identify a family of ideal 2D Dirac semimetals, which has nonzero Berry curvature in the vicinity of Dirac points and visible edge states, thus facilitating the experimental observations. Our work shows that 2D Dirac points can emerge without inversion symmetry, which not only enriches the classification of 2D topological semimetals but also provides a promising avenue to observe exotic transport phenomena beyond graphene, e.g., nonlinear Hall effect.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا