اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدUltrafast laser-induced changes of the magnetic anisotropy in a low-symmetry iron garnet film
183
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
We explore a thermal mechanism of changing the anisotropy by femtosecond laser pulses in dielectric ferrimagnetic garnets by taking a low symmetry (YBiPrLu)3(FeGa)5O12 film grown on the (210)-oriented Gd3Ga5O12 substrate as a model media. We demonstrate by means of spectral magneto-optical pump-probe technique and phenomenological analysis, that the magnetization precession in such a film is triggered by laser-induced changes of the growth-induced magnetic anisotropy along with the well-known ultrafast inverse Faraday effect. The change of magnetic anisotropy is mediated by the lattice heating induced by laser pulses of arbitrary polarization on a picosecond time scale. We show that the orientation of the external magnetic field with respect to the magnetization easy plane noticeably affects the precession excited via the anisotropy change. Importantly, the relative contributions from the ultrafast inverse Faraday effect and the change of different growth-induced anisotropy parameters can be controlled by varying the applied magnetic field strength and direction. As a result, the amplitude and the initial phase of the excited magnetization precession can be gradually tuned.
قيم البحث
اقرأ أيضاً
We use time-resolved x-ray resonant magnetic scattering (tr-XRMS) at the Co M$_{2,3}$- and Tb O$_1$-edges to study ultrafast demagnetization in an amorphous Co$_{88}$Tb$_{12}$ alloy with stripe domains. Combining the femtosecond temporal with nanomet
er spatial resolution of our experiment, we demonstrate that the equilibrium spin texture of the thin film remains unaltered by the optical pump-pulse on ultrashort timescales ($<$1 ps). However, after $simeq$ 4 ps, we observe the onset of a significant domain wall broadening, which we attribute to a reduction of the uniaxial magnetic anisotropy of the system, due to energy transfer to the lattice. Static temperature dependent magnetometry measurements combined with analytical modeling of the magnetic structure of the thin film corroborate this interpretation.
We use time-resolved molecular orbital mapping to explore fundamental processes of excited wave packets and charge transfer dynamics in organic films on femtosecond time scales. We investigate a bilayer pentacene film on Ag(110) by optical laser pump
and FEL probe experiments. From the angle-resolved photoemission signal, we obtain time-dependent momentum maps of the molecular valence states that can be related to their molecular initial states by simulations of the involved photoemission matrix elements. We discover a state above the Fermi edge that is temporarily occupied after optical excitation. The wave function of this state is imaged and identified as a transient charge transfer exciton extending over two neighboring molecules.
The response in capacitance to low external magnetic fields (up to 0.1 T) of suspensions of spherical magnetic nanoparticles, single-wall carbon nanotubes (SWCNT), SWCNT functionalized with carboxyl group (SWCNT-COOH) and SWCNT functionalized with Fe
$_3$O$_4$ nanoparticles in a nematic liquid crystal has been studied experimentally. The volume concentration of nanoparticles was $phi_1$ = 10$^{-4}$ and $phi_2$ = 10$^{-3}$. Independent of the type and the volume concentration of the nanoparticles, a linear response to low magnetic fields (far below the magnetic Freederiksz transition threshold) has been observed, which is not present in the undoped nematic.
Dynamical strain generated upon excitation of a metallic film by a femtosecond laser pulse may become a versatile tool enabling control of magnetic state of thin films and nanostructures via inverse magnetostriction on a picosecond time scale. Here w
e explore two alternative approaches to manipulate magnetocrystalline anisotropy and excite magnetization precession in a low-symmetry film of a magnetic metallic alloy galfenol (Fe,Ga) either by injecting picosecond strain pulse into it from a substrate or by generating dynamical strain of complex temporal profile in the film directly. In the former case we realize ultrafast excitation of magnetization dynamics solely by strain pulses. In the latter case optically-generated strain emerged abruptly in the film modifies its magnetocrystalline anisotropy, competing with heat-induced change of anisotropy parameters. We demonstrate that the optically-generated strain remains efficient for launching magnetization precession, when the heat-induced changes of anisotropy parameters do not trigger the precession anymore. We emphasize that in both approaches the ultrafast change of magnetic anisotropy mediating the precession excitation relies on mixed, compressive and shear, character of the dynamical strain, which emerges due to low-symmetry of the metallic film under study.
Laser induced ultrafast demagnetization in ferromagnetic metals was discovered almost 20 years ago, but currently there is still lack of consensus on the microscopic mechanism responsible for the corresponding transfer of angular momentum and energy
between electron, lattice and spin subsystems. A distinct, but intrinsically correlated phenomenon occurring on a longer timescale is the magnetization precession after the ultrafast demagnetization process, if a magnetic field is applied to tilt the magnetization vector away from its easy direction, which can be attributed to the change of anisotropy after laser heating. In an in-plane magnetized Pt/Co/Pt thin film with perpendicular interface anisotropy, we found excellent agreement between theoretical prediction with plausible parameters and experimental data measured using time resolved magneto-optical Kerr effect. This agreement confirms that the time evolution of the anisotropy field, which is driven by the interaction between electrons and phonons, determines the magnetization precession completely. A detailed analysis shows that, even though the whole sample is magnetized in-plane, the dynamic interface anisotropy field dictates the initial phase of the magnetization precession, highlighting the significance of the interface anisotropy field in laser induced magnetization precession.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
