Coexistence of Superconductivity and Magnetism in FeSe_1-x under Pressure

An extended investigation of the electronic phase diagram of FeSe$_{1-x}$ up to pressures of $psimeq2.4$,GPa by means of ac and dc magnetization, zero field muon spin rotation (ZF $mu$SR), and neutron diffraction is presented. ZF $mu$SR indicates that at pressures $pgeq0.8$,GPa static magnetic order occurs in FeSe$_{1-x}$ and occupies the full sample volume for $pgtrsim 1.2$,GPa. ac magnetization measurements reveal that the superconducting volume fraction stays close to 100% up to the highest pressure investigated. In addition, above $pgeq1.2$,GPa both the superconducting transition temperature $T_{rm c}$ and the magnetic ordering temperature $T_{rm N}$ increase simultaneously, and both superconductivity and magnetism are stabilized with increasing pressure. Calculations indicate only one possible muon stopping site in FeSe$_{1-x}$, located on the line connecting the Se atoms along the $c$-direction. Different magnetic structures are proposed and checked by combining the muon stopping calculations with a symmetry analysis, leading to a similar structure as in the LaFeAsO family of Fe-based superconductors. Furthermore, it is shown that the magnetic moment is pressure dependent and with a rather small value of $muapprox 0.2,mu_B$ at $psimeq2.4$,GPa.