اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدTweaking the spin-wave dispersion and suppressing the incommensurate phase in LiNiPO$_4$ by iron substitution
47
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
Elastic and inelastic neutron scattering studies of Li(Ni$_{1-x}$Fe$_{x}$)PO$_4$ single crystals reveal anomalous spin-wave dispersions along the crystallographic direction parallel to the characteristic wave vector of the magnetic incommensurate phase. The anomalous spin-wave dispersion ({it magnetic soft mode}) indicates the instability of the Ising-like ground state that eventually evolves into the incommensurate phase as the temperature is raised. The pure LiNiPO$_4$ system ($x=0$), undergoes a first-order magnetic phase transition from a long-range incommensurate phase to an antiferromagnetic ground state at {it T}$_N$ = 20.8 K. At 20% Fe concentrations, although the AFM ground state is to a large extent preserved as that of the pure system, the phase transition is second-order, and the incommensurate phase is completely suppressed. Analysis of the dispersion curves using a Heisenberg spin Hamiltonian that includes inter- and in-plane nearest and next-nearest neighbor couplings reveals frustration due to strong competing interactions between nearest- and a next-nearest neighbor site, consistent with the observed incommensurate structure. The Fe substitution only slightly lowers the extent of the frustration, sufficient to suppress the IC phase. An energy gap in the dispersion curves gradually decreases with the increase of Fe content from $sim$2 meV for the pure system ($x=0$) to $sim$0.9 meV for $x=0.2$.
قيم البحث
اقرأ أيضاً
Neutron diffraction with static and pulsed magnetic fields is used to directly probe the magnetic structures in LiNiPO$_4$ up to 25T and 42T, respectively. By combining these results with magnetometry and electric polarization measurements under puls
ed fields, the magnetic and magnetoelectric phases are investigated up to 56T applied along the easy $c$-axis. In addition to the already known transitions at lower fields, three new ones are reported at 37.6, 39.4 and 54T. Ordering vectors are identified with ${bf Q}_{mathrm{VI}}$ = (0, 1/3, 0) in the interval 37.6--39.4T and ${bf Q}_{mathrm{VII}}$ = (0, 0, 0) in the interval 39.4-54T. A quadratic magnetoelectric effect is discovered in the ${bf Q}_{mathrm{VII}}$ = (0, 0, 0) phase and the field-dependence of the induced electric polarization is described using a simple mean-field model. The observed magnetic structure and magnetoelectric tensor elements point to a change in the lattice symmetry in this phase. We speculate on the possible physical mechanism responsible for the magnetoelectric effect in LiNiPO4.
The magnetic structure for the newly discovered iron-arsenide compound CaFeAs has been studied by neutron powder diffraction. Long-range magnetic order is detected below 85K, with an incommensurate modulation described by the propagation vector k=(0,
$delta$,0), $deltasim$ 0.39. Below $sim$ 25K, our measurements detect a first-order phase transition where $delta$ locks into the commensurate value 3/8. A model of the magnetic structure is proposed for both temperature regimes, based on Rietveld refinements of the powder data and symmetry considerations. The structures correspond to longitudinal spin-density-waves with magnetic moments directed along the textit{b}-axis. A Landau analysis captures the change in thermodynamic quantities observed at the two magnetic transitions, in particular the drop in resistivity at the lock-in transition.
The presence of incommensurate spiral spin-density waves (SDW) has been proposed to explain the $p$ (hole doping) to $1+p$ jump measured in the Hall number $n_H$ at a doping $p^*$. Here we explore {it collinear} incommensurate SDW as another possible
explanation of this phenomenon, distinct from the incommensurate {it spiral} SDW proposal. We examine the effect of different SDW strengths and wavevectors and we find that the $n_Hsim p$ behavior is hardly reproduced at low doping. The calculated $n_H$ and Fermi surfaces give characteristic features that should be observed, thus the lack of these features in experiment suggests that the incommensurate collinear SDW is unlikely to be a good candidate to explain the $n_Hsim p$ observed in the pseudogap regime.
Recent neutron scattering measurements reveal spin and charge ordering in the half-doped nickelate, La$_{3/2}$ Sr$_{1/2}$ NiO$_4$. Many of the features of the magnetic excitations have been explained in terms of the spin waves of diagonal stripes wit
h weak single-ion anisotropy. However, an optical mode dispersing away from the (pi,pi) point was not captured by this theory. We show here that this apparent optical mode is a natural consequence of stripe twinning in a diagonal stripe pattern with a magnetic coupling structure which is two-fold symmetric, i.e. one possessing the same spatial rotational symmetry as the ground state.
We report magnetization, specific heat, and NMR measurements of 3-Br-4-F-V [=3-(3-bromo-4-fluorophenyl)-1,5-diphenylverdazyl], a strong-rung S=1/2 Heisenberg spin ladder with ferromagnetic leg interactions. We explain the magnetic and thermodynamic p
roperties based on the strong-rung regime. Furthermore, we find a field-induced successive phase transition in the specific heat and the nuclear spin-lattice relaxation rate 1/T1. 19F-NMR spectra for higher- and lower-temperature phases indicate partial magnetic order and incommensurate long-range order, respectively, evidencing the presence of frustration due to weak interladder couplings.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
