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The substitution of one metal ion in a Cr-based molecular ring with dominant antiferromagnetic couplings allows to engineer its level structure and ground-state degeneracy. Here we characterize a Cr7Ni molecular ring by means of low-temperature specific-heat and torque-magnetometry measurements, thus determining the microscopic parameters of the corresponding spin Hamiltonian. The energy spectrum and the suppression of the leakage-inducing S-mixing render the Cr7Ni molecule a suitable candidate for the qubit implementation, as further substantiated by our quantum-gate simulations.
Surfaces are at the frontier of every known solid. They provide versatile supports for functional nanostructures and mediate essential physicochemical processes. Being intimately related with 2D materials, interfaces and atomically thin films often f
Presented are magnetization measurements on a crystal of Cr7Ni antiferromagnetic rings. Irradiation with microwaves at frequencies between 1 and 10 GHz leads to observation of very narrow resonant photon absorption lines which are mainly broadened by
Bottom-up prepared carbon nanostructures appear as promising platforms for future carbon-based nanoelectronics, due to their atomically precise and versatile structure. An important breakthrough is the recent preparation of nanoporous graphene (NPG)
We outline a range of proposals on using quantum rings and nanohelices for terahertz device implementations. We show that an Aharonov-Bohm quantum ring system and a double-gated quantum ring system both permit control over the polarization properties
We demonstrated theoretically that a circularly polarized electromagnetic field substantially modifies electronic properties of a periodical chain of quantum rings. Particularly, the field opens band gaps in the electron energy spectrum of the chain,