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تسجيل مستخدم جديدPartially Diffusive Helium-Silica Compound in the Deep Interiors of Giant Planets
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Helium is the second most abundant element in the universe, and together with silica, they are major components of giant planets. Exploring the reactivity and state of helium and silica under high pressure is of fundamental importance for developing and understanding of the evolution and internal structure of giant planets. Here, using first-principles calculations and crystal structure predictions, we identify four stable phases of a helium-silica compound with seven/eight-coordinated silicon atoms at pressure range of 600-4000 GPa, corresponding to the interior condition of the outer planets in the solar system. The density of HeSiO2 agrees with current structure models of the planets. This helium-silica compound exhibits a superionic-like helium diffusive state at the high pressure and high temperature conditions along the isentropes of Saturn, a metallic fluid state in Jupiter, and a solid state in the deep interiors of Uranus and Neptune. The reaction of helium and silica may lead to the erosion of the rocky core of giant planets and form a diluted core region. These results highlight the reactivity of helium under high pressure to form new compounds, and also provides evidence to help build more sophisticated interior models of giant planets.
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Silica, water and hydrogen are known to be the major components of celestial bodies, and have significant influence on the formation and evolution of giant planets, such as Uranus and Neptune. Thus, it is of fundamental importance to investigate thei
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Changes in atomic coordination numbers at high pressures are fundamental to condensed-matter physics because they initiate the emergence of unexpected structures and phenomena. Silicon is capable of forming eight-, nine-, and ten-coordinated structur
es under compression,in addition to the usual six-coordinated structures. The missing seven-coordinated silicon remains an open question, but here our theoretical study provides evidence for its existence at high pressures. A combination of a crystal-structure prediction method and first-principles calculations allowed prediction of a stable SiO2He compound containing unique SiO7 polyhedrons, which is a configuration unknown in any proposed silica phase. Consequently, seven-coordinated SiO7 is a possible form of silica at high pressures. Further calculations indicate that the SiO2He phase remains energetically stable with a solid character over a wide range of pressures exceeding 607 GPa and temperatures of 0-9000 K, covering the extreme conditions of the core-mantle boundary in super-Earth exoplanets, or even the Solar Systems ice giant planets. Our results may provide theoretical guidance for the discovery of other silicides at high pressures, promote the exploration of materials at planetary core-mantle boundaries, and enable planetary models to be refined.
The sun and giant planets are generally thought to have the same helium abundance as that in the solar nebula from which they were formed 4.6 billion years ago. In contrast, the interstellar medium reflects current galactic conditions. The departure
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