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Frustration enhanced by Kitaev-exchange in a $boldsymbol{tilde{j}_{text{eff}}=frac12}$ triangular antiferromagnet

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 نشر من قبل Vladislav Kataev
 تاريخ النشر 2021
  مجال البحث فيزياء
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Triangular Heisenberg antiferromagnets are prototypes of geometric frustration, even if for nearest-neighbor interactions quantum fluctuations are not usually strong enough to destroy magnetic ordering: stronger frustration is required to stabilize a spin-liquid phase. On the basis of static magnetization and ESR measurements, we demonstrate the emergence of ${tilde{j}_{text{eff}}=frac12}$ moments in the triangular-lattice magnet Na$_2$BaCo(PO$_4$)$_2$. These moments are subject to an extra source of frustration that causes magnetic correlations to set in far above both the magnetic ordering and Weiss temperatures. Corroborating the $tilde{j}_{text{eff}}=frac12$ ground state, theory identifies ferromagnetic Kitaev exchange anisotropy as additional frustrating agent, altogether putting forward Na$_2$BaCo(PO$_4$)$_2$ as a new, promising Kitaev spin-liquid material.



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