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The exploitation of phonon-polaritons in nanostructured materials offers a pathway to manipulate infrared (IR) light for nanophotonic applications. Notably, hyperbolic phonons polaritons (HP2) in polar bidimensional crystals have been used to demonstrate strong electromagnetic field confinement, ultraslow group velocities, and long lifetimes (~ up to 8 ps). Here we present nanobelts of {alpha}-phase molybdenum trioxide ({alpha}-MoO3) as a low-dimensional medium supporting HP2 modes in the mid- and far-IR ranges. By real-space nanoimaging, with IR illuminations provided by synchrotron and tunable lasers, we observe that such HP2 response happens via formation of Fabry-Perot resonances. We remark an anisotropic propagation which critically depends on the frequency range. Our findings are supported by the convergence of experiment, theory, and numerical simulations. Our work shows that the low dimensionality of natural nanostructured crystals, like {alpha}-MoO3 nanobelts, provides an attractive platform to study polaritonic light-matter interactions and offer appealing cavity properties that could be harnessed in future designs of compact nanophotonic devices.
Hyperbolic phonon polaritons (HPhPs) in orthorhombic-phase molybdenum trioxide ($alpha$-MoO3) show in-plane hyperbolicity, great wavelength compression and ultra-long lifetime, therefore holding great potential in nanophotonic applications. However,
Surface phonon polaritons (SPhPs) in polar dielectrics offer new opportunities for infrared nanophotonics due to sub-diffraction confinement with low optical losses. Though the polaritonic field confinement can be significantly improved by modifying
Highly confined and low-loss hyperbolic phonon polaritons (HPhPs) sustained in van der Waals crystals exhibit outstanding capabilities of concentrating long-wave electromagnetic fields deep to the subwavelength region. Precise tuning on the HPhP prop
Hyperbolic phonon polaritons (HPhPs) sustained in van der Waals (vdW) materials exhibit extraordinary capabilities of confining long-wave electromagnetic fields to the deep subwavelength scale. In stark contrast to the uniaxial vdW hyperbolic materia
Moire engineering as a configuration method to twist van der Waals materials has delivered a series of advances in electronics, magnetics and optics. Yet these advances stem from peculiar moire superlattices which form at small specific twisting angl