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تسجيل مستخدم جديدImaging the atomic-scale electronic states induced by a pair of hole dopants in Ca2CuO2Cl2 Mott insulator
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We use scanning tunneling microscopy to visualize the atomic-scale electronic states induced by a pair of hole dopants in Ca2CuO2Cl2 parent Mott insulator of cuprates. We find that when the two dopants approach each other, the transfer of spectral weight from high energy Hubbard band to low energy in-gap state creates a broad peak and nearly V-shaped gap around the Fermi level. The peak position shows a sudden drop at distance around 4 a0 and then remains almost constant. The in-gap states exhibit peculiar spatial distributions depending on the configuration of the two dopants relative to the underlying Cu lattice. These results shed important new lights on the evolution of low energy electronic states when a few holes are doped into parent cuprates.
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Although the mechanism of superconductivity in the cuprates remains elusive, it is generally agreed that at the heart of the problem is the physics of doped Mott insulators. The cuprate parent compound has one unpaired electron per Cu site, and is pr
edicted by band theory to be a half-filled metal. The strong onsite Coulomb repulsion, however, prohibits electron hopping between neighboring sites and leads to a Mott insulator ground state with antiferromagnetic (AF) ordering. Charge carriers doped into the CuO2 plane destroy the insulating phase and superconductivity emerges as the carrier density is sufficiently high. The natural starting point for tackling high Tc superconductivity is to elucidate the electronic structure of the parent Mott insulator and the behavior of a single doped charge. Here we use a scanning tunneling microscope to investigate the atomic scale electronic structure of the Ca2CuO2Cl2 parent Mott insulator of the cuprates. The full electronic spectrum across the Mott-Hubbard gap is uncovered for the first time, which reveals the particle-hole symmetric and spatially uniform Hubbard bands. A single electron donated by surface defect is found to create a broad in-gap electronic state that is strongly localized in space with spatial characteristics intimately related to the AF spin background. The unprecedented real space electronic structure of the parent cuprate sheds important new light on the origion of high Tc superconductivity from the doped Mott insulator perspective.
Unusual transport properties of superconducting (SC) materials, such as the under doped cuprates, low dimensional superconductors in strong magnetic fields, and insulating films near the Insulator Superconductor Transition (IST), have been attributed
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When periodicity of crystal is disturbed by atomic disorder, its electronic state becomes inhomogeneous and band dispersion is obscured. In case of Fe-based superconductors, disorder of chalcogen/pnictogen height causes disorder of Fe 3d level splitt
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Because the cuprate superconductors are doped Mott insulators, it would be advantageous to solve even a toy model that exhibits both Mottness and superconductivity. We consider the Hatsugai-Kohmoto model, an exactly solvable system that is a prototyp
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We present a systematic study of spin dynamics in a superconducting ground state, which itself is a doped-Mott-insulator and can correctly reduce to an antiferromagnetic (AF) state at half-filling with an AF long-range order (AFLRO). Such a doped Mot
t insulator is described by a mean-field theory based on the phase string formulation of the t-J model. We show that the spin wave excitation in the AFLRO state at half-filling evolves into a resonancelike peak at a finite energy in the superconducting state, which is located around the AF wave vectors. The width of such a resonancelike peak in momentum space decides a spin correlation length scale which is inversely proportional to the square root of doping concentration, while the energy of the resonancelike peak scales linearly with the doping concentration at low doping. An important prediction of the theory is that, while the total spin sum rule is satisfied at different doping concentrations, the weight of the resonancelike peak does not vanish, but is continuously saturated to the weight of the AFLRO at zero-doping limit. Besides the low-energy resonancelike peak, we also show that the high-energy excitations still track the spin wave dispersion in momentum space, contributing to a significant portion of the total spin sum rule. The fluctuational effect beyond the mean-field theory is also examined, which is related to the broadening of the resonancelike peak in energy space. In particular, we discuss the incommensurability of the spin dynamics by pointing out that its visibility is strongly tied to the low-energy fluctuations below the resonancelike peak. We finally investigate the interlayer coupling effect on the spin dynamics as a function of doping, by considering a bilayer system.
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