ترغب بنشر مسار تعليمي؟ اضغط هنا

Nonlinear optical conductivity of a two-band crystal I

54   0   0.0 ( 0 )
 نشر من قبل Daniel Passos
 تاريخ النشر 2021
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

The structure of the electronic nonlinear optical conductivity is elucidated in a detailed study of the time-reversal symmetric two-band model. The nonlinear conductivity is decomposed as a sum of contributions related with different regions of the First Brillouin Zone, defined by single or multiphoton resonances. All contributions are written in terms of the same integrals, which contain all information specific to the particular model under study. In this way, ready-to-use formulas are provided that reduce the often tedious calculations of the second and third order optical conductivity to the evaluation of a small set of similar integrals. In the scenario where charge carriers are present prior to optical excitation, Fermi surface contributions must also be considered and are shown to have an universal frequency dependence, tunable by doping. General characteristics are made evident in this type of resonance-based analysis: the existence of step functions that determine the chemical potential dependence of electron-hole symmetric insulators; the determination of the imaginary part by Hilbert transforms, simpler than those of the nonlinear Kramers-Kr{o}nig relations; the absence of Drude peaks in the diagonal elements of the second order conductivity, among others. As examples, analytical expressions are derived for the nonlinear conductivities of some simple systems: a very basic model of direct gap semiconductors and the Dirac fermions of monolayer graphene.

قيم البحث

اقرأ أيضاً

Motivated by developments in quantum information science, much recent effort has been directed toward coupling individual quantum emitters to optical microcavities. Such systems can be used to produce single photons on demand, enable nonlinear optica l switching at a single photon level, and implement functional nodes of a quantum network, where the emitters serve as processing nodes and photons are used for long-distance quantum communication. For many of these practical applications, it is important to develop techniques that allow one to generate outgoing single photons of desired frequency and bandwidth, enabling hybrid networks connecting different types of emitters and long-distance transmission over telecommunications wavelengths. Here, we propose a novel approach that makes use of a nonlinear optical resonator, in which the single photon originating from the atom-like emitter is directly converted into a photon with desired frequency and bandwidth using the intracavity nonlinearity. As specific examples, we discuss a high-finesse, TE-TM double-mode photonic crystal cavity design that allows for direct generation of single photons at telecom wavelengths starting from an InAs/GaAs quantum dot with a 950 nm transition wavelength, and a scheme for direct optical coupling of such a quantum dot with a diamond nitrogen-vacancy center at 637 nm.
Following our ab initio nonlinear optical (NLO) materials design guidelines, in this Letter, we discovered a novel type of structure to realize potential deep-ultraviolet (DUV) NLO performance in the classical beryllium borate system. By densely stac king the NLO-active layered frameworks, the key design scheme for the structural evolution from the (Be2BO3F2) layers in KBe2BO3F2 (KBBF) to the novel (Be2BO5H3) layers in berborite is illustrated. Based on available experimental results and systematical theoretical evaluation from first principles, the NLO properties of berborite are further obtained as comparable as the only pratical DUV NLO crystal KBBF. It is demonstrated that berborite can achieve available DUV phase-matched output with strong NLO effect for the practically important 177.3 nm and 193.7 nm lasers. Once obtained with sizable single crystal, it can be applied as a promising DUV NLO crystal.
42 - Zoran Rukelj , Ana Akrap 2021
Here we study the single-particle, electronic transport and optical properties of a gapped system described by a simple two-band Hamiltonian with inverted valence bands. We analyze its properties in the three-dimensional (3D) and the two-dimensional (2D) case. The insulating phase changes into a metallic phase when the band gap is set to zero. The metallic phase in the 3D case is characterized by a nodal surface. This nodal surface is equivalent to a nodal ring in two dimensions. Within a simple theoretical framework, we calculate the density of state, the total and effective charge carrier concentration, the Hall concentration and the Hall coefficient, for both 2D and 3D cases. The main result is that the three concentrations always differ from one another in the present model. These concentrations can then be used to resolve the nature of the electronic ground state. Similarly, the optical conductivity is calculated and discussed for the insulating phase. We show that there are no optical excitations in the metallic phase. Finally, we compare the calculated optical conductivity with the rule-of-thumb derivation using the joint density of states.
Recent studies have emphasized the importance of impurity scattering for the optical Higgs response of superconductors. In the dirty limit, an additional paramagnetic coupling of light to the superconducting condensate arises which drastically enhanc es excitation. So far, most work concentrated on the periodic driving with light, where the third-harmonic generation response of the Higgs mode was shown to be enhanced. In this work, we additionally calculate the time-resolved optical conductivity of single- and two-band superconductors in a two-pulse quench-probe setup, where we find good agreement with existing experimental results. We use the Mattis-Bardeen approach to incorporate impurity scattering and calculate explicitly the time-evolution of the system. Calculations are performed both in a diagrammatic picture derived from an effective action formalism and within a time-dependent density matrix formalism.
We theoretically show how two impurity defects in a crystalline structure can be entangled through coupling with the crystal. We demonstrate this with a harmonic chain of trapped ions in which two ions of a different species are embedded. Entanglemen t is found for sufficiently cold chains and for a certain class of initial, separable states of the defects. It results from the interplay between localized modes which involve the defects and the interposed ions, it is independent of the chain size, and decays slowly with the distance between the impurities. These dynamics can be observed in systems exhibiting spatial order, viable realizations are optical lattices, optomechanical systems, or cavity arrays in circuit QED.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا