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Eutectic gallium-indium (EGaIn), a room-temperature liquid metal alloy, has the largest tension of any liquid at room temperature, and yet can nonetheless undergo fingering instabilities. This effect arises because, under an applied voltage, oxides deposit on the surface of the metal, which leads to a lowering of the interfacial tension, allowing spreading under gravity. Understanding the spreading dynamics of room temperature liquid metals is important for developing soft electronics and understanding fluid dynamics of liquids with extreme surface tensions. When the applied voltage or the oxidation rate becomes too high, the EGaIn undergoes fingering instabilities, including tip-splitting, which occur due to a Marangoni stress on the interface. Our experiments are performed with EGaIn droplets placed in an electrolyte (sodium hydroxide); by placing the EGaIn on copper electrodes, which EGaIn readily wets, we are able to control the initial width of EGaIn fingers, setting the initial conditions of the spreading. Two transitions are observed: (1) a minimum current density at which all fingers become unstable to narrower fingers; (2) a current density at which the wider fingers undergo a single splitting event into two narrower fingers. We present a phase diagram as a function of current density and initial finger width, and identify the minimum width below which the single tip-splitting does not occur.
Marangoni propulsion is a form of locomotion wherein an asymmetric release of surfactant by a body located at the surface of a liquid leads to its directed motion. We present in this paper a mathematical model for Marangoni propulsion in the viscous
Marangoni instabilities can emerge when a liquid interface is subjected to a concentration or temperature gradient. It is generally believed that for these instabilities bulk effects like buoyancy are negligible as compared to interfacial forces, esp
In this paper, the interfacial motion between two immiscible viscous fluids in the confined geometry of a Hele-Shaw cell is studied. We consider the influence of a thin wetting film trailing behind the displaced fluid, which dynamically affects the p
We consider the creeping flow of a Newtonian fluid in a hemispherical region. In a domain with spherical, or nearly spherical, geometry, the solution of Stokes equation can be expressed as a series of spherical harmonics. However, the original Lamb s
Surface coatings and patterning technologies are essential for various physicochemical applications. In this Letter, we describe key parameters to achieve uniform particle coatings from binary solutions: First, multiple sequential Marangoni flows, se