اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدSingle-Hemisphere Photoelectron Momentum Microscope With Time-of-Flight Recording
146
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
Photoelectron momentum microscopy is an emerging powerful method for angle-resolved photoelectron spectroscopy (ARPES), especially in combination with imaging spin filters. These instruments record kx-ky images, typically exceeding a full Brillouin zone. As energy filters double-hemispherical or time-of-flight (ToF) devices are in use. Here we present a new approach for momentum mapping of the full half-space, based on a single hemispherical analyzer (path radius 225 mm). Excitation by an unfocused He lamp yielded an energy resolution of 7.7 meV. The performance is demonstrated by k-imaging of quantum-well states in Au and Xe multilayers. The alpha-square-aberration term (alpha: entrance angle in the dispersive plane) and the transit-time spread of the electrons in the spherical field are studied in a large pass-energy (6 to 660 eV) and angular range (alpha up to about 7{deg}). It is discussed how the method circumvents the preconditions of previous theoretical work on the resolution limitation due to the alpha-square-term and the transit-time spread, being detrimental for time-resolved experiments. Thanks to k-resolved detection, both effects can be corrected numerically. We introduce a dispersive-plus-ToF hybrid mode of operation, with an imaging ToF analyzer behind the exit slit of the hemisphere. This instrument captures 3D data arrays I(EB,kx,ky), yielding a gain up to N^2 in recording efficiency (N being the number of resolved time slices). A key application will be ARPES at sources with high pulse rates like Synchrotrons with 500 MHz time structure.
قيم البحث
اقرأ أيضاً
Since the MICROSCOPE instrument aims to measure accelerations as low as a few 10$^{-15}$,m,s$^{-2}$ and cannot operate on ground, it was obvious to have a large time dedicated to its characterization in flight. After its release and first operation,
the characterization experiments covered all the aspects of the instrument design in order to consolidate the scientific measurements and the subsequent conclusions drawn from them. Over the course of the mission we validated the servo-control and even updated the PID control laws for each inertial sensor. Thanks to several dedicated experiments and the analysis of the instrument sensitivities, we have been able to identify a number of instrument characteristics such as biases, gold wire and electrostatic stiffnesses, non linearities, couplings and free motion ranges of the test-masses, which may first impact the scientific objective and secondly the analysis of the instrument good operation.
We report here a general theory describing photoelectron transportation dynamics in GaAs semiconductor photocathodes. Gradient doping is incorporated in the model through the inclusion of directional carrier drift. The time-evolution of electron conc
entration in the active layer upon the injection of an excitation pulse is solved both numerically and analytically. The predictions of the model are compared with experiments via carrier-induced transient reflectivity change, which is measured for gradient-doped and uniform-doped photocathodes using femtosecond pump-probe reflectometry. Excellent agreement is found between the experiments and the theory, leading to the characterization of key device parameters such as diffusion constant and electron decay rates. Comparisons are also made between uniform doping and gradient doping for their characteristics in photoelectron transportation. Doping gradient is found to be able to accelerate electron accumulation on the device surface. These results offer new insights into the dynamics of III-V photocathodes and potentially open a new avenue toward experimental characterization of device parameters.
The sensing of magnetic fields has important applications in medicine, particularly to the sensing of signals in the heart and brain. The fields associated with biomagnetism are exceptionally weak, being many orders of magnitude smaller than the Eart
hs magnetic field. To measure them requires that we use the most sensitive detection techniques, however, to be commercially viable this must be done at an affordable cost. The current state of the art uses costly SQUID magnetometers, although they will likely be superseded by less costly, but otherwise limited, alkali vapour magnetometers. Here, we discuss the application of diamond magnetometers to medical applications. Diamond magnetometers are robust, solid state devices that work in a broad range of environments, with the potential for sensitivity comparable to the leading technologies.
We demonstrate that photoemission properties of GaAs photocathodes (PCs) can be altered by surface acoustic waves (SAWs) generated on the PC surface due to dynamical piezoelectric fields of SAWs. Simulations with COMSOL indicate that electron effecti
ve lifetime in p-doped GaAs may increase by a factor of 10x to 20x. It implies a significant, by a factor of 2x to 3x, increase of quantum efficiency (QE) for GaAs PCs. Essential steps in device fabrication are demonstrated, including deposition of an additional layer of ZnO for piezoelectric effect enhancement, measurements of I-V characteristic of the SAW device, and ability to survive high-temperature annealing.
Vertically stacked atomic layers from different layered crystals can be held together by van der Waals forces, which can be used for building novel heterostructures, offering a platform for developing a new generation of atomically thin, transparent
and flexible devices. The performance of these devices is critically dependent on the layer thickness and the interlayer electronic coupling, influencing the hybridisation of the electronic states as well as charge and energy transfer between the layers. The electronic coupling is affected by the relative orientation of the layers as well as by the cleanliness of their interfaces. Here, we demonstrate an efficient method for monitoring interlayer coupling in heterostructures made from transition metal dichalcogenides using photoluminescence imaging in a bright-field optical microscope. The colour and brightness in such images are used here to identify mono- and few-layer crystals, and to track changes in the interlayer coupling and the emergence of interlayer excitons after thermal annealing in mechanically exfoliated flakes as well as a function of the twist angle in atomic layers grown by chemical vapour deposition. Material and crystal thickness sensitivity of the presented imaging technique makes it a powerful tool for characterisation of van der Waals heterostructures assembled by a wide variety of methods, using combinations of materials obtained through mechanical or chemical exfoliation and crystal growth.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
