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Sliding and twisting van der Waals layers with respect to each other gives rise to moire structures with emergent electronic properties. Electrons in these moire structures feel weak potentials that are typically in the tens of millielectronvolt range when the moire structures are smooth at the atomic scale. Here we report a facile technique to achieve deep, deterministic trapping potentials via strain-based moire engineering in van der Waals bilayers. We use elasto-scanning tunneling microscopy to show that uniaxial strain drives a commensurate-incommensurate lattice transition in a multilayer MoSe$_2$ system. In the incommensurate state, the top monolayer is partially detached from the bulk through the spontaneous formation of topological solitons where stress is relieved. Intersecting solitons form a honeycomb-like network resulting from the three-fold symmetry of the adhesion potential between layers. The vertices of the honeycomb network occur in bound pairs with different interlayer stacking arrangements. One vertex of the pair is found to be an efficient trap for electrons, displaying two states that are deeply confined within the semiconductor gap and have a spatial extent of 2 nm. Honeycomb soliton networks thus provide a unique path to engineer an array of identical deeply confined states with a strain-dependent tunable spatial separation, without the necessity of introducing chemical defects into the host materials.
Two-dimensional (2D) materials exhibit a number of improved mechanical, optical, electronic properties compared to their bulk counterparts. The absence of dangling bonds in the cleaved surfaces of these materials allows combining different 2D materia
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Stacking monolayers of transition metal dichalcogenides into a heterostructure with a finite twist-angle gives rise to artificial moire superlattices with a tunable periodicity. As a consequence, excitons experience a periodic potential, which can be
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Layered materials can be assembled vertically to fabricate a new class of van der Waals (VDW) heterostructures a few atomic layers thick, compatible with a wide range of substrates and optoelectronic device geometries, enabling new strategies for con