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Coupling different physical properties is a fascinating subject of physics. Already well-known are the multiferroics which show properties of ferroelectrics and magnets. But ferroelectricity by itself also entails the bulk photovoltaic effect, a light-matter interaction which generates dc currents. Here we propose a magnetic photogalvanic effect that couples the magnetism to the light-matter interaction. This phenomenon emerges from the $mathbf{k}$ to $mathbf{-k}$ symmetry-breaking in the band structure and does not require a static polarization. It is distinct from other known bulk photovoltaic mechanisms such as the shift current. We demonstrate such phenomena in a newly discovered layered magnetic insulator CrI$_3$. A record photoconductivity response (more than 200 $mu A V^{-2} $) is generated under the irradiation of a visible light in the antiferromagnetic phase. The current can be reversed and switched by controllable magnetic phase transitions. Our work paves a new route for photovoltaic and optoelectronic devices and provides a sensitive probe for the magnetic transition.
The optical properties of transition metal dichalcogenide monolayers are widely dominated by excitons, Coulomb-bound electron-hole pairs. These quasi-particles exhibit giant oscillator strength and give rise to narrow-band, well-pronounced optical tr
Magnetic phase transitions often occur spontaneously at specific critical temperatures. The presence of more than one critical temperature (Tc) has been observed in several compounds where the coexistence of competing magnetic orders highlights the i
Higher-order exchange interactions and quantum effects are widely known to play an important role in describing the properties of low-dimensional magnetic compounds. Here we identify the recently discovered two-dimensional (2D) van der Waals (vdW) Cr
Polarization, denoting the precession direction with respect to the background magnetization, is an intrinsic degree of freedom of spin wave. Using magnetic textures to control the spin wave polarization is fundamental and indispensable toward reprog
Merons are nontrivial topological spin textures highly relevant for many phenomena in solid state physics. Despite their importance, direct observation of such vortex quasiparticles is scarce and has been limited to a few complex materials. Here we s