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Ultrafast processes in matter can be captured and even controlled by using sequences of few-cycle optical pulses, which need to be well characterized, both in amplitude and phase. The same degree of control has not yet been achieved for few-cycle extreme ultraviolet pulses generated by high-order harmonic generation in gases, with duration in the attosecond range. Here, we show that by varying the spectral phase and carrier-envelope phase (CEP) of a high-repetition rate laser, using dispersion in glass, we achieve a high degree of control of the relative phase and CEP between consecutive attosecond pulses. The experimental results are supported by a detailed theoretical analysis based upon the semiclassical three-step model for high-order harmonic generation.
We study the photoionization of argon atoms close to the 3s$^2$3p$^6$ $rightarrow$ 3s$^1$3p$^6$4p $leftrightarrow$ 3s$^2$3p$^5$ $varepsilon ell$, $ell$=s,d Fano window resonance. An interferometric technique using an attosecond pulse train, i.e. a fr
We study the higher-harmonic generation (HHG) using elliptically polarized two-color driving fields. The HHG via bi-chromatic counter-rotating laser fields is a promising source of circularly polarized ultrashort XUV radiation at the attosecond time
The recent development of ultrafast extreme ultraviolet (XUV) coherent light sources bears great potential for a better understanding of the structure and dynamics of matter. Promising routes are advanced coherent control and nonlinear spectroscopy s
Resonant enhancement of high harmonic generation can be obtained in plasmas containing ions with strong radiative transitions resonant with harmonic orders. The mechanism for this enhancement is still debated. We perform the first temporal characteri
Trains of ultrashort laser pulses separated by the time of rotational revival (typically, tens of picoseconds) have been exploited for creating ensembles of aligned molecules. In this work we introduce a chiral pulse train - a sequence of linearly po