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A consistent view of the samarium hexaboride terminations to resolve the nature of its surface states

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 نشر من قبل Emile Rienks
 تاريخ النشر 2018
  مجال البحث فيزياء
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The research effort prompted by the prediction that SmB$_6$ could be the first topological Kondo insulator has produced a wealth of new results, though not all of these seem compatible. A major discrepancy exists between scanning tunneling microscopy / spectroscopy (STM/S) and angle-resolved photoemission spectroscopy (ARPES), because the two experimental methods suggest a very different number of terminations of the (100) surface with different properties. Here we tackle this issue in a combined STM/S and ARPES study. We find that two of the well-ordered topographies reported in earlier STM studies can be associated with the crystal terminations identified using photoemission. We further observe a reversal of the STM contrast with bias voltage for one of the topographies. We ascribe this result to a different energy dependence of Sm and B-derived states, and show that it can be used to obtain element specific images of SmB$_6$ and identify which topography belongs to which termination. We finally find STS results to support a modification of the low-energy electronic structure at the surface that has been proposed as the trivial origin of surface metallicity in this material.



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The recent conjecture of a topologically-protected surface state in SmB$_6$ and the verification of robust surface conduction below 4 K have prompted a large effort to understand the surface states. Conventional Hall transport measurements allow curr ent to flow on all surfaces of a topological insulator, so such measurements are influenced by contributions from multiple surfaces of varying transport character. Instead, we study magnetotransport of SmB$_6$ using a Corbino geometry, which can directly measure the conductivity of a single, independent surface. Both (011) and (001) crystal surfaces show a strong negative magnetoresistance at all magnetic field angles measured. The (011) surface has a carrier mobility of $122text{ cm}^2/text{V}cdottext{sec}$ with a carrier density of $2.5times10^{13} text{ cm}^{-2}$, which are significantly smaller than indicated by Hall transport studies. This mobility value can explain a failure so far to observe Shubnikov-de Haas oscillations. Analysis of the angle-dependence of conductivity on the (011) surface suggests a combination of a field-dependent enhancement of the carrier density and a suppression of Kondo scattering from native oxide layer magnetic moments as the likely origin of the negative magnetoresistance. Our results also reveal a hysteretic behavior whose magnitude depends on the magnetic field sweep rate and temperature. Although this feature becomes smaller when the field sweep is slower, does not disappear or saturate during our slowest sweep-rate measurements, which is much slower than a typical magnetotransport trace. These observations cannot be explained by quantum interference corrections such as weak anti-localization, but are more likely due to an extrinsic magnetic effect such as the magnetocaloric effect or glassy ordering.
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