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Spin dynamics and field-induced magnetic phase transition in the honeycomb Kitaev magnet ${alpha}$-Li$_2$IrO$_3$

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 نشر من قبل Radu Coldea
 تاريخ النشر 2018
  مجال البحث فيزياء
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The layered honeycomb iridate $alpha$-Li$_2$IrO$_3$ displays an incommensurate magnetic structure with counterrotating moments on nearest-neighbor sites, proposed to be stabilized by strongly-frustrated anisotropic Kitaev interactions between spin-orbit entangled Ir$^{4+}$ magnetic moments. Here we report powder inelastic neutron scattering measurements that observe sharply dispersive low-energy magnetic excitations centered at the magnetic ordering wavevector, attributed to Goldstone excitations of the incommensurate order, as well as an additional intense mode above a gap $Deltasimeq2.3$ meV. Zero-field muon-spin relaxation measurements show clear oscillations in the muon polarization below the N{e}el temperature $T_{rm N}simeq15$ K with a time-dependent profile consistent with bulk incommensurate long-range magnetism. Pulsed field magnetization measurements observe that only about half the saturation magnetization value is reached at the maximum field of 64 T. A clear anomaly near 25 T indicates a transition to a phase with reduced susceptibility. The transition field has a Zeeman energy comparable to the zero-field gapped mode, suggesting gap suppression as a possible mechanism for the field-induced transition.



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