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The passage of time is tracked by counting oscillations of a frequency reference, such as Earths revolutions or swings of a pendulum. By referencing atomic transitions, frequency (and thus time) can be measured more precisely than any other physical quantity, with the current generation of optical atomic clocks reporting fractional performance below the $10^{-17}$ level. However, the theory of relativity prescribes that the passage of time is not absolute, but impacted by an observers reference frame. Consequently, clock measurements exhibit sensitivity to relative velocity, acceleration and gravity potential. Here we demonstrate optical clock measurements surpassing the present-day ability to account for the gravitational distortion of space-time across the surface of Earth. In two independent ytterbium optical lattice clocks, we demonstrate unprecedented levels in three fundamental benchmarks of clock performance. In units of the clock frequency, we report systematic uncertainty of $1.4 times 10^{-18}$, measurement instability of $3.2 times 10^{-19}$ and reproducibility characterised by ten blinded frequency comparisons, yielding a frequency difference of $[-7 pm (5)_{stat} pm (8)_{sys}] times 10^{-19}$. While differential sensitivity to gravity could degrade the performance of these optical clocks as terrestrial standards of time, this same sensitivity can be used as an exquisite probe of geopotential. Near the surface of Earth, clock comparisons at the $1 times 10^{-18}$ level provide 1 cm resolution along gravity, outperforming state-of-the-art geodetic techniques. These optical clocks can further be used to explore geophysical phenomena, detect gravitational waves, test general relativity and search for dark matter.
We evaluated the static and dynamic polarizabilities of the 5s^2 ^1S_0 and 5s5p ^3P_0^o states of Sr using the high-precision relativistic configuration interaction + all-order method. Our calculation explains the discrepancy between the recent exper
Atomic clocks have been transformational in science and technology, leading to innovations such as global positioning, advanced communications, and tests of fundamental constant variation. Next-generation optical atomic clocks can extend the capabili
Quantum non-demolition (QND) measurement is a remarkable tool for the manipulation of quantum systems. It allows specific information to be extracted while still preserving fragile quantum observables of the system. Here we apply cavity-based QND mea
We use a quantum non-demolition measurement to generate a spin squeezed state and to create entanglement in a cloud of 10^5 cold cesium atoms, and for the first time operate an atomic clock improved by spin squeezing beyond the projection noise limit
Optical frequency comparison of the 40Ca+ clock transition u_{Ca} (2S1/2-2D5/2, 729nm) against the 87Sr optical lattice clock transition u_{Sr}(1S0-3P0, 698nm) has resulted in a frequency ratio u_{Ca} / u_{Sr} = 0.957 631 202 358 049 9(2 3). The