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We report detailed dc and ac magnetic susceptibilities, specific heat, and thermal conductivity measurements on the frustrated magnet ZnCr$_2$Se$_4$. At low temperatures, with increasing magnetic field, this spinel material goes through a series of spin state transitions from the helix spin state to the spiral spin state and then to the fully polarized state. Our results indicate a direct quantum phase transition from the spiral spin state to the fully polarized state. As the system approaches the quantum criticality, we find strong quantum fluctuations of the spins with the behaviors such as an unconventional $T^2$-dependent specific heat and temperature independent mean free path for the thermal transport. We complete the full phase diagram of ZnCr$_2$Se$_4$ under the external magnetic field and propose the possibility of frustrated quantum criticality with extended densities of critical modes to account for the unusual low-energy excitations in the vicinity of the criticality. Our results reveal that ZnCr$_2$Se$_4$ is a rare example of 3D magnet exhibiting a field-driven quantum criticality with unconventional properties.
Muon spin rotation/relaxation spectroscopy %(supported by magnetization measurements) has been employed to study electron localization around a donor center - the positive muon - in the 3d magnetic spinel semiconductor CdCr$_2$Se$_4$ at temperatures
In the spinel compound GeCo$_2$O$_4$, the Co$^{2+}$ pyrochlore sublattice presents remarkable magnetic field-induced behaviors that we unveil through neutron and X-ray single-crystal diffraction. The Neel ordered magnetic phase is entered through a s
We report pressure-dependent reflection and transmission measurements on ZnCr$_2$Se$_4$, HgCr$_2$S$_4$, and CdCr$_2$O$_4$ single crystals at room temperature over a broad spectral range 200-24000 cm$^{-1}$. The pressure dependence of the phonon modes
We demonstrate via a muon spin rotation experiment that the electronic ground state of the iridium spinel compound, CuIr$_2$S$_4$, is not the presumed spin-singlet state but a novel paramagnetic state, showing a quasistatic spin glass-like magnetism
The frustrated magnet SrDy$_2$O$_4$ exhibits a field-induced phase with a magnetization plateau at $1/3$ of the saturation value for magnetic fields applied along the $b$-axis. We report here a neutron scattering study of the nature and symmetry of t