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We probe dephasing mechanisms within a quantum network node consisting of a single nitrogen-vacancy centre electron spin that is hyperfine coupled to surrounding $^{13} text{C}$ nuclear-spin quantum memories. Previous studies have analysed memory dephasing caused by the stochastic electron-spin reset process, which is a component of optical internode entangling protocols. Here, we find, by using dynamical decoupling techniques and exploiting phase matching conditions in the electron-nuclear dynamics, that control infidelities and quasi-static noise are the major contributors to memory dephasing induced by the entangling sequence. These insights enable us to demonstrate a 19-fold improved memory performance which is still not limited by the electron reinitialization process. We further perform pump-probe studies to investigate the spin-flip channels during the optical electron spin reset. We find that spin-flips occur via decay from the meta-stable singlet states with a branching ratio of 8(1):1:1, in contrast with previous work. These results allow us to formulate straightforward improvements to diamond-based quantum networks and similar architectures.
Spin echo techniques are essential for achieving long coherence times in solid-state quantum memories for light because of inhomogeneous broadening of the spin transitions. It has been suggested that unrealistic levels of precision for the radio freq
We demonstrate operation of a rotation sensor based on the $^{14}$N nuclear spins intrinsic to nitrogen-vacancy (NV) color centers in diamond. The sensor employs optical polarization and readout of the nuclei and a radio-frequency double-quantum puls
A rotation sensor is one of the key elements of inertial navigation systems and compliments most cellphone sensor sets used for various applications. Currently, inexpensive and efficient solutions are mechanoelectronic devices, which nevertheless lac
With the ability to transfer and process quantum information, large-scale quantum networks will enable a suite of fundamentally new applications, from quantum communications to distributed sensing, metrology, and computing. This perspective reviews r
Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be rapidly pola